APPLICATION OF THE SUM-FREQUENCY GENERATION TO THE VIBRATIONAL SPECTROSCOPY OF A LANGMUIR-BLODGETT-FILM

被引：8
|
作者：
PFLUMIO, V
VALLET, JC
BOEGLIN, AJ
VILLAEYS, AA
LAVOINE, JP
机构：
[1] Institut de Physique et Chimie des Matériaux de Strasbourg, Groupe d'Optique Nonlinéaire et d'Optoélectronique, CR 67037 Strasbourg-Cedex, 23, rue du Loess
来源：
PHYSICAL REVIEW A | 1995年 / 51卷 / 04期
关键词：
D O I：
10.1103/PhysRevA.51.3174
中图分类号：
O43 [光学];
学科分类号：
070207 ; 0803 ;
摘要：
In this paper, we calculate the sum-frequency generation (SFG) signal for molecules adsorbed on a surface. The expression is established as a function of the molecular microscopic constants and for different polarization combinations of the input beams. Next, this result is applied to reproduce simultaneously experimental SFG spectra of pentadecanoic acid molecules on a water surface obtained for different polarizations of the input beams. From the fit, we have been able to determine unambiguously the microscopic parameters of the adsorbate. © 1995 The American Physical Society.
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收藏
页码：3174 / 3181
页数：8
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