Greenhouse gases emissions in rivers of the Tibetan Plateau

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作者
Bin Qu
Kelly Sue Aho
Chaoliu Li
Shichang Kang
Mika Sillanpää
Fangping Yan
Peter A. Raymond
机构
[1] Yale-NUIST Center on Atmospheric Environment,Department of Civil and Environmental Engineering
[2] International Joint Laboratory on Climate and Environment Change (ILCEC),undefined
[3] Nanjing University of Information Science and Technology,undefined
[4] Laboratory of Green Chemistry,undefined
[5] Lappeenranta University of Technology,undefined
[6] Key Laboratory of Tibetan Environment Changes and Land Surface Processes,undefined
[7] Institute of Tibetan Plateau Research,undefined
[8] Chinese Academy of Sciences,undefined
[9] Yale School of Forestry and Environmental Studies,undefined
[10] Yale University,undefined
[11] CAS Center for Excellence in Tibetan Plateau Earth Sciences,undefined
[12] Chinese Academy of Sciences,undefined
[13] State Key Laboratory of Cryospheric Science,undefined
[14] Northwest Institute of Eco-Environmental and resources,undefined
[15] Chinese Academy of Sciences,undefined
[16] University of Chinese Academy of Sciences,undefined
[17] Florida International University,undefined
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摘要
Greenhouse gases (GHGs) emissions from streams are important to regional biogeochemical budgets. This study is one of the first to incorporate stream GHGs (CO2, CH4 and N2O) concentrations and emissions in rivers of the Tibetan Plateau. With one-time sampling from 32 sites in rivers of the plateau, we found that most of the rivers were supersaturated with CO2, CH4 and N2O during the study period. Medians of partial pressures of CO2 (pCO2), pCH4 and pN2O were presented 864 μatm, 6.3 μatm, and 0.25 μatm respectively. Based on a scaling model of the flux of gas, the calculated fluxes of CO2, CH4 and N2O (3,452 mg-C m2 d−1, 26.7 mg-C m2 d−1 and 0.18 mg-N m2 d−1, respectively) in rivers of the Tibetan Plateau were found comparable with most other rivers in the world; and it was revealed that the evasion rates of CO2 and CH4 in tributaries of the rivers of the plateau were higher than those in the mainstream despite its high altitude. Furthermore, concentrations of GHGs in the studied rivers were related to dissolved carbon and nitrogen, indicating that riverine dissolved components could be used to scale GHGs envision in rivers of the Tibetan Plateau.
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