A broken translational symmetry state in an infinite-layer nickelate

被引:0
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作者
Matteo Rossi
Motoki Osada
Jaewon Choi
Stefano Agrestini
Daniel Jost
Yonghun Lee
Haiyu Lu
Bai Yang Wang
Kyuho Lee
Abhishek Nag
Yi-De Chuang
Cheng-Tai Kuo
Sang-Jun Lee
Brian Moritz
Thomas P. Devereaux
Zhi-Xun Shen
Jun-Sik Lee
Ke-Jin Zhou
Harold Y. Hwang
Wei-Sheng Lee
机构
[1] Stanford Institute for Materials and Energy Sciences,Department of Materials Science and Engineering
[2] SLAC National Accelerator Laboratory,Department of Applied Physics
[3] Stanford University,Department of Physics
[4] Diamond Light Source,Advanced Light Source
[5] Harwell Campus,Geballe Laboratory for Advanced Materials
[6] Stanford University,undefined
[7] Stanford University,undefined
[8] Lawrence Berkeley National Laboratory,undefined
[9] Stanford Synchrotron Radiation Lightsource,undefined
[10] SLAC National Accelerator Laboratory,undefined
[11] Stanford University,undefined
来源
Nature Physics | 2022年 / 18卷
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摘要
A defining signature of strongly correlated electronic systems is a rich phase diagram, which consists of multiple broken symmetries, such as magnetism, superconductivity and charge order1,2. In the recently discovered nickelate superconductors3–10, a large antiferromagnetic exchange energy has been reported, which implies the existence of strong electronic correlations11. However, signatures of a broken-symmetry state other than superconductivity have not yet been observed. Here we observe charge ordering in infinite-layer nickelates La1−xSrxNiO2 using resonant X-ray scattering. The parent compound orders along the Ni–O bond direction with an incommensurate wavevector, distinct from the stripe order observed in other nickelates12–14 that propagates along a direction 45° to the Ni–O bond. The resonance profile we measure indicates that ordering originates from the nickelate layers and induces a parasitic charge modulation of lanthanum electrons. Upon doping, the charge order diminishes and its wavevector shifts towards commensurate, hinting that strong electronic correlations are likely to be responsible for the ordered state. Our results suggest that the existence of charge order and its potential interplay with antiferromagnetic fluctuations and superconductivity are important themes in nickel-based superconductors.
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页码:869 / 873
页数:4
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