On the determination of 36Cl and 129I in solid materials from nuclear decommissioning activities

被引:0
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作者
Inés Llopart-Babot
Mirela Vasile
Andrew Dobney
Sven Boden
Michel Bruggeman
Martine Leermakers
Jixin Qiao
Phil Warwick
机构
[1] SCK CEN,Department of Environmental and Resource Engineering
[2] VUB,National Oceanography Centre
[3] AMGC,undefined
[4] Technical University of Denmark,undefined
[5] University of Southampton,undefined
关键词
Cl; I; Pyrolyser; Cl-resin; LSC; Nuclear decommissioning;
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摘要
Determination of the 36Cl and 129I massic activities using pyrolysis combined with radiochemical separation (using a Cl-resin) in concrete and graphite samples from decommissioning waste originating from Belgian Reactor 3 and 1 (SCK CEN, Belgium), respectively, is described. Liquid scintillation counting is used for their quantification. The chemical recovery of the procedure was evaluated by determining the stable chlorine with ion chromatography and stable iodine with inductively coupled plasma mass spectrometry. The method was optimized and verified by spiking inactive solid materials.
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页码:3313 / 3326
页数:13
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