Fabrication of UiO-66/g-C3N4 Heterostructure Nanocatalyst for Efficient Visible-Light Photocatalytic Performance

被引:9
|
作者
Xu, Shichao [1 ]
Yang, Weijing [2 ]
Liu, Yufan [1 ]
Yang, Jie [2 ]
Zu, Tongtong [1 ]
Hao, Mengchen [1 ]
Li, Yang [2 ]
Xiao, Yichen [2 ]
机构
[1] TianGong Univ, Sch Environm Sci & Engn, Tianjin 300389, Peoples R China
[2] TianGong Univ, Sch Chem, Tianjin 300389, Peoples R China
基金
中国国家自然科学基金;
关键词
Photodegradation; visible light; MOFs; g-C3N4; DEGRADATION; HETEROJUNCTION; EVOLUTION;
D O I
10.1142/S2251237322500022
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
It is well known that synthetic heterojunction photocatalysts can promote photocatalytic activity. Herein, we successfully combine UiO-66 with g-C3N4 as ultrathin layer coating via a convenient synthesis method, the photocatalytic performance through the degradation of RhB is then shown efficient. The heterojunction and high surface area give the photocatalysts an ability to promote visible light absorption and strengthen the separation and migration of photogenerated electrons, which ultimately leads to the improvement of photocatalytic degradation. The heterostructure nanocatalyst helps the degradation rate of RhB reach 98.98% in 140 min under visible light irradiation. In addition, the hole (h(+)) plays a major role in the reaction. This work offers an efficient method for the application in the field of environmental degradation.
引用
收藏
页数:9
相关论文
共 50 条
  • [1] Visible light photocatalytic degradation of MB using UiO-66/g-C3N4 heterojunction nanocatalyst
    Zhang, Ying
    Zhou, Jiabin
    Feng, Qinqin
    Chen, Xin
    Hu, Zeshu
    CHEMOSPHERE, 2018, 212 : 523 - 532
  • [2] g-C3N4/UiO-66 nanohybrids with enhanced photocatalytic activities for the oxidation of dye under visible light irradiation
    Zhang, Xiaodong
    Yang, Yang
    Huang, Wenyuan
    Yang, Yiqiong
    Wang, Yuxin
    He, Chi
    Liu, Ning
    Wu, Minghong
    Tang, Liang
    MATERIALS RESEARCH BULLETIN, 2018, 99 : 349 - 358
  • [3] Hydrothermal fabrication of α-SnWO4/g-C3N4 heterostructure with enhanced visible-light photocatalytic activity
    Liang, Qian
    Jin, Jie
    Liu, Changhai
    Xu, Song
    Yao, Chao
    Chen, Zhidong
    Li, Zhongyu
    JOURNAL OF MATERIALS SCIENCE-MATERIALS IN ELECTRONICS, 2017, 28 (15) : 11279 - 11283
  • [4] Hydrothermal fabrication of α-SnWO4/g-C3N4 heterostructure with enhanced visible-light photocatalytic activity
    Qian Liang
    Jie Jin
    Changhai Liu
    Song Xu
    Chao Yao
    Zhidong Chen
    Zhongyu Li
    Journal of Materials Science: Materials in Electronics, 2017, 28 : 11279 - 11283
  • [5] Enhanced visible-light photocatalytic performance of BiOBr/UiO-66(Zr) composite for dye degradation with the assistance of UiO-66
    Sha, Zhou
    Wu, Jishan
    RSC ADVANCES, 2015, 5 (49) : 39592 - 39600
  • [6] Fabrication of pyrimidine/g-C3N4 nanocomposites for efficient photocatalytic activity under visible-light illumination
    Zhuang, Jingguo
    Zhang, Jing
    Pang, Jingyu
    Wang, Aijian
    Wang, Xinhai
    Zhu, Weihua
    DYES AND PIGMENTS, 2019, 163 : 634 - 640
  • [7] Fabrication of porous g-C3N4 and supported porous g-C3N4 by a simple precursor pretreatment strategy and their efficient visible-light photocatalytic activity
    Zeng, Zhenxing
    Li, Kexin
    Wei, Kai
    Dai, Yuhua
    Yan, Liushui
    Guo, Huiqin
    Luo, Xubiao
    CHINESE JOURNAL OF CATALYSIS, 2017, 38 (03) : 498 - 508
  • [8] Construction of highly efficient g-C3N4/rutin heterostructure for enhanced photocatalytic performance under visible light
    Zhang, Shikang
    Yin, Haiyang
    Liu, Zhenchun
    MATERIALS LETTERS, 2022, 309
  • [9] Enhanced photocatalytic performance of ternary g-C3N4/UiO-66/Ag3VO4 composite for methylene blue degradation under visible light irradiation
    Meskelu, Kalkidan
    Taddesse, Abi M.
    Teju, Endale
    Bezu, Zewdu
    RESULTS IN CHEMISTRY, 2024, 11
  • [10] Heterojunction of UiO-66 and porous g-C3N4 for boosted photocatalytic removal of organic dye
    Lan, Dawei
    Zhu, Huiwen
    Zhang, Jianwen
    Xie, Chengrui
    Wang, Fan
    Zheng, Yueying
    Guo, Zeyu
    Xu, Mengxia
    Wu, Tao
    APPLIED SURFACE SCIENCE, 2024, 655