Critical Review of Eutrophication Models for Life Cycle Assessment

被引:78
|
作者
Morelli, Ben [1 ]
Hawkins, Troy R. [1 ,6 ]
Niblick, Briana [2 ]
Henderson, Andrew D. [2 ,7 ]
Golden, Heather E. [3 ]
Compton, Jana E. [4 ]
Cooter, Ellen J. [5 ]
Bare, Jane C. [2 ]
机构
[1] Franklin Associates, Eastern Res Grp, 110 Hartwell Ave, Lexington, MA 02421 USA
[2] US EPA, Natl Risk Management Res Lab, 26 West Martin Luther King Dr, Cincinnati, OH 45268 USA
[3] US EPA, Natl Exposure Res Lab, 26 West Martin Luther King Dr, Cincinnati, OH 45268 USA
[4] US EPA, Natl Hlth & Environm Effects Res Lab, 200 SW 35th St, Corvallis, OR 97333 USA
[5] US EPA, Natl Exposure Res Lab, 109 TW Alexander Dr, Res Triangle Pk, NC 27709 USA
[6] Argonne Natl Lab, 9700 Cass Ave, Lemont, IL 60439 USA
[7] Noblis Inc, 16414 San Pedro Ave,Suite 400, San Antonio, TX 78232 USA
关键词
MARINE EUTROPHICATION; NITROGEN INPUTS; POWER-PLANTS; FRESH-WATER; PHOSPHORUS; EMISSIONS; LAKE; NOX; SENSITIVITY; DEPOSITION;
D O I
10.1021/acs.est.8b00967
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
This paper evaluates the current state of life cycle impact assessment (LCIA) methods used to estimate potential eutrophication impacts in freshwater and marine ecosystems and presents a critical review of the underlying surface water quality, watershed, marine, and air fate and transport (F&T) models. Using a criteria rubric, we assess the potential of each method and model to contribute to further refinements of life cycle assessment (LCA) eutrophication mechanisms and nutrient transformation processes as well as model structure, availability, geographic scope, and spatial and temporal resolution. We describe recent advances in LCIA modeling and provide guidance on the best available sources of fate and exposure factors, with a focus on midpoint indicators. The critical review identifies gaps in LCIA characterization modeling regarding the availability and spatial resolution of fate factors in the soil compartment and identifies strategies to characterize emissions from soil. Additional opportunities are identified to leverage detailed F&T models that strengthen existing approaches to LCIA or that have the potential to link LCIA modeling more closely with the spatial and temporal realities of the effects of eutrophication.
引用
收藏
页码:9562 / 9578
页数:17
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