Coherent Control of Angular Momentum Transfer in Resonant Two-Photon Light-Matter Interaction

被引：7
|
作者：
Malik, D. A. [1 ]
Kimel, A. V. [1 ]
Kirilyuk, A. [1 ]
Rasing, Th. [1 ]
van der Zande, W. J. [1 ]
机构：
[1] Radboud Univ Nijmegen, Inst Mol & Mat, NL-6500 GL Nijmegen, Netherlands
来源：
PHYSICAL REVIEW LETTERS | 2010年 / 104卷 / 13期
关键词：
MAGNETISM; PULSES; TRANSITIONS;
D O I：
10.1103/PhysRevLett.104.133001
中图分类号：
O4 [物理学];
学科分类号：
0702 ;
摘要：
We show experimentally and theoretically that a polarization-shaped femtosecond laser pulse with a zero net angular momentum creates a net angular momentum in atomic rubidium during resonant two-photon excitation. The necessary conditions for the creation of a nonzero angular momentum as well as the excitation efficiencies are analyzed in the framework of second-order time-dependent perturbation theory.
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页数：4
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