Intrinsic anomalous Hall effect in thin films of topological kagome ferromagnet Fe3Sn2

被引:13
|
作者
Khan, Kacho Imtiyaz Ali [1 ]
Yadav, Ram Singh [1 ]
Bangar, Himanshu [1 ]
Kumar, Akash [1 ]
Chowdhury, Niru [1 ]
Muduli, Prasanta Kumar [2 ]
Muduli, Pranaba Kishor [1 ]
机构
[1] Indian Inst Technol Delhi, Dept Phys, New Delhi 110016, India
[2] Indian Inst Technol Madras, Dept Phys, Chennai 600036, Tamil Nadu, India
关键词
INTERMETALLIC COMPOUNDS; CRYSTAL-STRUCTURE; LATTICE;
D O I
10.1039/d2nr00443g
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Fe3Sn2, a kagome ferromagnet, is a potential quantum material with intriguing topological features. Despite substantial experimental work on the bulk single crystals, the thin film growth of Fe3Sn2 remains relatively unexplored. Here, we investigate the effect of two different seed layers (Ta and Pt) on the growth of Fe3Sn2 thin films. We demonstrate the growth of polycrystalline Fe3Sn2 thin films on Si/SiO2 substrates by room temperature sputter deposition, followed by in situ annealing at 500 degrees C. Our structural and magnetic measurements indicate that a pure ferromagnetic phase is formed for the Pt/Fe3Sn2 thin films with higher saturation magnetization of M-s = 464 emu cc(-1), while a mixed-phase (consisting of ferromagnetic, Fe3Sn2 and antiferromagnetic, FeSn) is formed for the Ta/Fe3Sn2 thin films with a lower M-s of 240 emu cc(-1). The Pt/Fe3Sn2 thin films also exhibit an anomalous Hall coefficient, R-s approximate to 2.6 x 10(-10) omega cm(-1) G(-1) at room temperature, which is two order of magnitude higher compared to 3d-transition metal ferromagnets. A non-zero temperature-independent anomalous Hall conductivity sigma int(xy) = (23 +/- 11) omega(-1) cm(-1) indicates an intrinsic mechanism of anomalous Hall effect originating from Berry curvature. These results are important for realizing novel topological spintronic devices on a CMOS-compatible substrate.
引用
收藏
页码:8484 / 8492
页数:9
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