Separation of U (VI) ions from the aqueous phase onto polyphenol silica nanocomposite in the batch adsorption system

被引:16
|
作者
Mahmoud, Mohamed Ahmed [1 ,2 ]
机构
[1] Jazan Univ, Coll Engn, Dept Chem Engn, Jazan, Saudi Arabia
[2] Nucl Mat Author, Cairo, Egypt
关键词
U (VI); Polyphenol; Sorption: Nanocomposite; Recycling;
D O I
10.1016/j.aej.2021.02.044
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The chemical modified silica nanoparticles with a polyphenol compound were synthesized as a sorbent nanocomposite for U (VI) removal from the aqueous phase. The prepared Pyrogallol silica nanocomposite (PSCN) was described by some specific analysis. The experiments were carried out in a batch system. The maximum sorption capacity of the nanocomposite reached 58.45 mg/g at optimum operating conditions (sorption time 50 min, pH 5, dose 0.2 g, 100 mg/l of U (VI) and 30 degrees C). The sorption procedure was an exothermic system and the results were in good agreement with pseudo-second-order (R-2 > 99) and Langmuir isotherm (R-2 > 97). Regeneration and recycling studies indicate that the prepared nanocomposite has good effectiveness for up to five cycles. (C) 2021 THE AUTHORS. Published by Elsevier BV on behalf of Faculty of Engineering, Alexandria University. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/ licenses/by-nc-nd/4.0/).
引用
收藏
页码:3819 / 3827
页数:9
相关论文
共 50 条
  • [1] Adsorption of U(VI) ions on biotite from aqueous solutions
    Lee, Seung Yeop
    Baik, Min Hoon
    Lee, Yong Jae
    Lee, Young Boo
    APPLIED CLAY SCIENCE, 2009, 46 (03) : 255 - 259
  • [2] Adsorption of U(VI) onto kaolin studied by batch method
    Zhang, Hongxia
    Liu, Zhi
    Hu, Peizhuo
    Liu, Tonghuan
    Wu, Wangsuo
    JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2013, 298 (01) : 611 - 619
  • [3] Adsorption of U(VI) onto kaolin studied by batch method
    Hongxia Zhang
    Zhi Liu
    Peizhuo Hu
    Tonghuan Liu
    Wangsuo Wu
    Journal of Radioanalytical and Nuclear Chemistry, 2013, 298 : 611 - 619
  • [4] BATCH ADSORPTION OF Zn(II) IONS FROM AQUEOUS SOLUTION ONTO SAWDUST
    Nacu, Gabriela
    Negrila, Lacramioara
    Bulgariu, Laura
    REVUE ROUMAINE DE CHIMIE, 2017, 62 (4-5) : 439 - 447
  • [5] Adsorption of U(VI) from dilute aqueous solutions onto peat moss
    Omar, H. A.
    Aziz, M.
    Shakir, K.
    RADIOCHIMICA ACTA, 2007, 95 (01) : 17 - 24
  • [6] Adsorption of U(VI) ions from aqueous solution using nanogoethite powder
    Zhang, Lijiang
    Zhang, Xiaowen
    Lu, Qian
    Wu, Xiaoyan
    Jiang, Tianjiao
    Mi, Li
    Peng, Ying
    ADSORPTION SCIENCE & TECHNOLOGY, 2019, 37 (1-2) : 113 - 126
  • [7] Adsorption of U(VI) from Aqueous Solution onto Hydrotalcite-Like Compounds
    Nguyen Van Suc
    E-JOURNAL OF CHEMISTRY, 2012, 9 (02) : 669 - 679
  • [8] Adsorption of U (VI) ions from aqueous solution using silicon dioxide nanopowder
    Mahmoud, Mohamed Ahmed
    JOURNAL OF SAUDI CHEMICAL SOCIETY, 2018, 22 (02) : 229 - 238
  • [9] Amidoxime-functionalized magnetic graphene oxide-silica particles for adsorption of U(VI) ions from an aqueous medium
    Gulay Bayramoglu
    Ayse Gul Cimen
    Mehmet Yakup Arica
    Journal of Radioanalytical and Nuclear Chemistry, 2024, 333 : 585 - 597
  • [10] Amidoxime-functionalized magnetic graphene oxide-silica particles for adsorption of U(VI) ions from an aqueous medium
    Bayramoglu, Gulay
    Cimen, Ayse Gul
    Arica, Mehmet Yakup
    JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY, 2024, 333 (01) : 585 - 597