Simultaneous removal of NOx and SO2 from coal boiler flue gases by DC corona discharge ammonia radical shower systems:: pilot plant tests

被引:69
|
作者
Chang, JS
Urashima, K
Tong, YX
Liu, WP
Wei, HY
Yang, FM
Liu, XJ
机构
[1] McMaster Univ, Dept Engn Phys, Hamilton, ON L8S 4M1, Canada
[2] State Environm Protect Gen Agcy, Safety & Environm Protect Res Inst, Wuhan, Peoples R China
关键词
non-thermal plasma; flow stabilized corona discharge; radical injection; coal boiler flue gases; NOx and SO2; ammonia radical; flue gas;
D O I
10.1016/S0304-3886(02)00168-7
中图分类号
TM [电工技术]; TN [电子技术、通信技术];
学科分类号
0808 ; 0809 ;
摘要
Pilot scale tests were conducted for simultaneous removal of NOx and SO2 from coal boiler flue gases by corona discharge induced ammonia radical injection techniques, i.e. the corona radical shower system. Tests were conducted for the flue gas rate from 1000 to 1500 Nm(3)/h, the gas temperature from 62degreesC to 80degreesC, the ammonia-to-total acid gas molecule ratio from 0.88 to 1.3, applied voltage from 0 to 25 kV and NO initial concentration from 53 to 93 ppm. for a fixed SO2 of 800 ppm. The results show that SO2 removal increases with increasing ammonia radical injection rate and non-monotonically depends on in-put electrical power. The NOx removal increases with increasing in-put electrical power and ammonia radical injection rate. Approximately 9 kg Of SO2 were removed by 1 kWh of energy input with 99% Of SO2 removal, while approximately 125 g of NOx was removed by 1 kWh of energy input with 75% of removal efficiency. (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:313 / 323
页数:11
相关论文
共 50 条
  • [1] Experimental investigation on activating water vapor and ammonia by DC corona discharge radical shower technology for removal of SO2 from flue gases
    Jie, L
    Ming, S
    Yan, W
    Shang, KF
    Wang, NH
    Li, GF
    JOURNAL OF ADVANCED OXIDATION TECHNOLOGIES, 2004, 7 (02) : 146 - 153
  • [2] Study on the reactive characteristics of simultaneous removal of SO2 and NOx by corona discharge radical shower system
    Wu, Zu-Liang
    Gao, Xiang
    Li, Ji-Wu
    Sun, Pei-De
    Luo, Zhong-Yang
    Cen, Ke-Fa
    2008, Zhejiang University Press, 20 Yugu Road, Hangzhou, 310027, China (22):
  • [3] SIMULTANEOUS REMOVAL OF NOX AND SO2 FROM FLUE-GASES
    不详
    BRENNSTOFF-WARME-KRAFT, 1987, 39 (11): : 478 - 478
  • [4] Removal of SO2 and NOx from flue gases by a new type of high freqency corona brush discharge
    Miljevic, V
    APPLIED PHYSICS IN SERBIA-APS, 2002, : 213 - 215
  • [5] Effects of Water Vapor and Ammonia on SO2 Removal from Flue Gases using Pulsed Corona Discharge
    Yimin Z.
    Chae J.O.
    Kim K.Y.
    Kim K.O.
    Park Y.K.
    Plasma Chemistry and Plasma Processing, 2002, 22 (01) : 187 - 195
  • [6] SO2 removal from industrial flue gases using pulsed corona discharge
    Wu, Y
    Wang, NH
    Zhu, YM
    Zhang, YB
    JOURNAL OF ELECTROSTATICS, 1998, 44 (1-2) : 11 - 16
  • [7] Electric discharge removal of SO2 and NOx from combustion flue gas by pulsed corona discharge
    Toyohashi Univ of Technology, Aichi, Japan
    Energy Convers Manage, 10-13 (1377-1387):
  • [8] Removal of SO2 from flue gas by water vapor DC corona discharge
    Division of Basic Courses, Shanghai Maritime University, Shanghai 200135, China
    不详
    Huanjing Kexue, 2006, 7 (1282-1285):
  • [9] Electric discharge removal of SO2 and NOx from combustion flue gas by pulsed corona discharge
    Onda, K
    Kasuga, Y
    Kato, K
    Fujiwara, M
    Tanimoto, M
    ENERGY CONVERSION AND MANAGEMENT, 1997, 38 (10-13) : 1377 - 1387
  • [10] Simultaneous removal of NOx and SO2 from NO-SO2-CO2-N2-O2 gas mixtures by corona radical shower systems
    Park, JY
    Tomicic, I
    Round, GF
    Chang, JS
    JOURNAL OF PHYSICS D-APPLIED PHYSICS, 1999, 32 (09) : 1006 - 1011