Catalytic partial oxidation (CPOX) of natural gas and renewable hydrocarbons/oxygenated hydrocarbons-A review

被引:53
|
作者
Ma, Ruoshui [1 ,2 ]
Xu, Bang [3 ]
Zhang, Xiao [1 ,2 ]
机构
[1] Washington State Univ, Voiland Sch Chem Engn & Bioengn, 2710 Crimson Way, Richland, WA 99354 USA
[2] Pacific Northwest Natl Lab, 2710 Crimson Way, Richland, WA 99354 USA
[3] Dason Technol, 3100 George Washington Way,S108, Richland, WA 99354 USA
关键词
Partial oxidation; Natural Gas; Reforming; Catalysis; Renewable; PEROVSKITE-TYPE OXIDES; METHANE PARTIAL OXIDATION; FLUIDIZED-BED REACTOR; HYDROGEN-PRODUCTION; OXYGEN-CARRIER; CARBON-MONOXIDE; SELECTIVE OXIDATION; FUEL-CELLS; BIO-OIL; BIOMASS GASIFICATION;
D O I
10.1016/j.cattod.2019.06.025
中图分类号
O69 [应用化学];
学科分类号
081704 ;
摘要
Catalytic partial oxidation (CPOX) is one of the most promising technologies for converting natural gas for fuel and chemicals synthesis. CPOX has been gaining increasing attention for conversion of natural gas to ideal syngas mixtures for fuel production. The urgency and importance of this endeavour has been increasingly recognized in the last few years due to the exploration of shale gas and flare gas. However, the information regarding the progress of industrial implementation of this technology is scarce. This review presents recent advances of CPOX techniques from bench to pilot scale and a comparison of its energy efficiency, carbon conversion efficiency, and operating costs with parallel technologies including steam reforming (SMR), autothermal reforming (ATR), and partial oxidation (POX). The potential applications and perspective of CPOX for long chain hydrocarbon and renewable hydrocarbon/oxygenated hydrocarbons conversion to new platform chemical and materials is also discussed.
引用
收藏
页码:18 / 30
页数:13
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