共 50 条
Dry Particulate Nitrate Deposition in China
被引:26
|作者:
Liu, Lei
[1
]
Zhang, Xiuying
[1
]
Zhang, Yan
[2
]
Xu, Wen
[3
]
Liu, Xuejun
[3
]
Zhang, Xiaomin
[1
,4
]
Feng, Junlan
[2
]
Chen, Xinrui
[2
]
Zhang, Yuehan
[5
]
Lu, Xuehe
[1
]
Wang, Shanqian
[1
]
Zhang, Wuting
[1
]
Zhao, Limin
[1
]
机构:
[1] Nanjing Univ, Int Inst Earth Syst Sci, Jiangsu Prov Key Lab Geog Informat Sci & Technol, Nanjing 210023, Jiangsu, Peoples R China
[2] Fudan Univ, Dept Environm Sci & Engn, Ctr Atmospher Chem Study, Shanghai 200433, Peoples R China
[3] China Agr Univ, Coll Resources & Environm Sci, Ctr Resources Environm & Food Secur, Key Lab Plant Soil Interact MOE, Beijing 100193, Peoples R China
[4] Jiangsu Ctr Collaborat Innovat Geog Informat Reso, Nanjing 210023, Jiangsu, Peoples R China
[5] Nanjing Univ, Sch Atmospher Sci, Nanjing 200433, Jiangsu, Peoples R China
基金:
中国国家自然科学基金;
关键词:
NITROGEN DEPOSITION;
CHEMICAL-COMPOSITIONS;
MATTER FORMATION;
GLOBAL MONSOON;
NO2;
AEROSOLS;
TRENDS;
MODEL;
EXCHANGE;
PM2.5;
D O I:
10.1021/acs.est.7b00898
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
A limited number of ground measurements of dry particulate nitrate deposition (NO3-) makes it difficult and challenging to fully know the status of the spatial and temporal variations of dry NO3- depositions over China. This study tries to expand the ground measurements of NO3- concentrations at monitoring sites to a national scale, based on the Ozone Monitoring Instrument (OMI) NO2 columns, NO2 profiles from an atmospheric chemistry transport model (Model for Ozone and Related chemical Tracers, version 4, MOZART-4) and monitor-based sources, and then estimates the NO3- depositions on a regional scale based on an inferred model. The ground NO2 concentrations were first derived from NO2 columns and the NO2 profiles, and then the ground NO3- concentrations were derived from the ground NO2 concentrations and the relationship between NO2 and NO3- based on Chinese Nationwide Nitrogen Deposition Monitoring Network (NNDMN). This estimated dry NO3- depositions over China will be helpful in determining the magnitude and pollution status in regions without ground measurements, supporting the construction plan of environmental monitoring in future.
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页码:5572 / 5581
页数:10
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