Dry Particulate Nitrate Deposition in China

被引:26
|
作者
Liu, Lei [1 ]
Zhang, Xiuying [1 ]
Zhang, Yan [2 ]
Xu, Wen [3 ]
Liu, Xuejun [3 ]
Zhang, Xiaomin [1 ,4 ]
Feng, Junlan [2 ]
Chen, Xinrui [2 ]
Zhang, Yuehan [5 ]
Lu, Xuehe [1 ]
Wang, Shanqian [1 ]
Zhang, Wuting [1 ]
Zhao, Limin [1 ]
机构
[1] Nanjing Univ, Int Inst Earth Syst Sci, Jiangsu Prov Key Lab Geog Informat Sci & Technol, Nanjing 210023, Jiangsu, Peoples R China
[2] Fudan Univ, Dept Environm Sci & Engn, Ctr Atmospher Chem Study, Shanghai 200433, Peoples R China
[3] China Agr Univ, Coll Resources & Environm Sci, Ctr Resources Environm & Food Secur, Key Lab Plant Soil Interact MOE, Beijing 100193, Peoples R China
[4] Jiangsu Ctr Collaborat Innovat Geog Informat Reso, Nanjing 210023, Jiangsu, Peoples R China
[5] Nanjing Univ, Sch Atmospher Sci, Nanjing 200433, Jiangsu, Peoples R China
基金
中国国家自然科学基金;
关键词
NITROGEN DEPOSITION; CHEMICAL-COMPOSITIONS; MATTER FORMATION; GLOBAL MONSOON; NO2; AEROSOLS; TRENDS; MODEL; EXCHANGE; PM2.5;
D O I
10.1021/acs.est.7b00898
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A limited number of ground measurements of dry particulate nitrate deposition (NO3-) makes it difficult and challenging to fully know the status of the spatial and temporal variations of dry NO3- depositions over China. This study tries to expand the ground measurements of NO3- concentrations at monitoring sites to a national scale, based on the Ozone Monitoring Instrument (OMI) NO2 columns, NO2 profiles from an atmospheric chemistry transport model (Model for Ozone and Related chemical Tracers, version 4, MOZART-4) and monitor-based sources, and then estimates the NO3- depositions on a regional scale based on an inferred model. The ground NO2 concentrations were first derived from NO2 columns and the NO2 profiles, and then the ground NO3- concentrations were derived from the ground NO2 concentrations and the relationship between NO2 and NO3- based on Chinese Nationwide Nitrogen Deposition Monitoring Network (NNDMN). This estimated dry NO3- depositions over China will be helpful in determining the magnitude and pollution status in regions without ground measurements, supporting the construction plan of environmental monitoring in future.
引用
收藏
页码:5572 / 5581
页数:10
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