Antibunching Single-Photon Emission and Blinking Suppression of CdSe/ZnS Quantum Dots

被引:78
|
作者
Yuan, C. T.
Yu, Pyng
Ko, H. C.
Huang, J.
Tang, Jau [1 ]
机构
[1] Acad Sinica, Res Ctr Appl Sci, Taipei 115, Taiwan
关键词
blinking suppression; single-photon emission; photon antibunching; CdSe/ZnS quantum dots; FLUORESCENCE; MOLECULE;
D O I
10.1021/nn900760u
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We demonstrated that by property coupling to silver nanoprisms, single CdSe/ZnS semiconductor quantum dots (QDs) exhibited suppressed blinking behavior, an enhanced fluorescence intensity (similar to 2.5 fold), increased radiative decay rates (similar to 12.5,fold), and antibunching single-photon emission. All these modifications significantly promote the overall performance of the proposed single-photon sources based on colloidal semiconductor QDs.
引用
收藏
页码:3051 / 3056
页数:6
相关论文
共 50 条
  • [1] Colloidal CdSe/ZnS quantum dots as single-photon sources
    Brokmann, X
    Messin, G
    Desbiolles, P
    Giacobino, E
    Dahan, M
    Hermier, JP
    NEW JOURNAL OF PHYSICS, 2004, 6 : 1 - 8
  • [2] Photon antibunching in single CdSe/ZnS quantum dot fluorescence
    Lounis, B
    Bechtel, HA
    Gerion, D
    Alivisatos, P
    Moerner, WE
    CHEMICAL PHYSICS LETTERS, 2000, 329 (5-6) : 399 - 404
  • [3] Blinking Suppression in CdSe/ZnS Single Quantum Dots by TiO2 Nanoparticles
    Hamada, Morihiko
    Nakanishi, Shunsuke
    Itoh, Tamitake
    Ishikawa, Mitsuru
    Biju, Vasudevanpillai
    ACS NANO, 2010, 4 (08) : 4445 - 4454
  • [4] Blueing, bleaching, and blinking of single CdSe/ZnS quantum dots
    van Sark, WGJHM
    Frederix, PLTM
    Bol, AA
    Gerritsen, HC
    Meijerink, A
    CHEMPHYSCHEM, 2002, 3 (10) : 871 - 879
  • [5] Blinking Suppression and Anti-Bunching of Quantum Dots as Single-Photon Sources
    Yu, Pyng
    Yuan, Chi-Tsu
    Ko, Hsien-Chien
    Huang, Jane
    Tang, Jau
    QUANTUM SENSING AND NANOPHOTONIC DEVICES VII, 2010, 7608
  • [6] Photon Antibunching in Small Clusters of CdSe/ZnS Core/Shell Quantum Dots
    Whitcomb, Kevin J.
    Geisenhoff, Jessica Q.
    Ryan, Duncan P.
    Gelfand, Martin P.
    Van Orden, Alan
    JOURNAL OF PHYSICAL CHEMISTRY B, 2015, 119 (29): : 9020 - 9028
  • [7] Blinking suppression of colloidal CdSe/ZnS quantum dots by coupling to silver nanoprisms
    Yuan, C. T.
    Yu, Pyng
    Tang, Jau
    APPLIED PHYSICS LETTERS, 2009, 94 (24)
  • [8] Single-photon emission of CdSe quantum dots at temperatures up to 200 K
    Sebald, K
    Michler, P
    Passow, T
    Hommel, D
    Bacher, G
    Forchel, A
    APPLIED PHYSICS LETTERS, 2002, 81 (16) : 2920 - 2922
  • [9] Antibunching and blinking from a single colloidal CdSe quantum dot
    Xu XingSheng
    Chen Shuai
    Yamada, Toshiki
    SCIENCE CHINA-PHYSICS MECHANICS & ASTRONOMY, 2010, 53 (09) : 1619 - 1625
  • [10] Antibunching and blinking from a single colloidal CdSe quantum dot
    YAMADA Toshiki
    Science China(Physics,Mechanics & Astronomy), 2010, (09) : 1619 - 1625