Tetramethylammonium hydroxide production using the microbial electrolysis desalination and chemical-production cell

被引：21

作者：

Liu, Guangli ^{[1
]}

Luo, Haiping ^{[1
]}

Tang, Yaobo ^{[1
]}

Chen, Shanshan ^{[1
]}

Zhang, Renduo ^{[1
]}

Hou, Yanping ^{[1
]}

机构：

[1] Sun Yat Sen Univ, Sch Environm Sci & Engn, Guangdong Prov Key Lab Environm Pollut Control &, Guangzhou 510275, Guangdong, Peoples R China

来源：

CHEMICAL ENGINEERING JOURNAL | 2014年 / 258卷

基金：

中国国家自然科学基金;

关键词：

Tetramethylammonium hydroxide; Bioelectrochemical system; Energy consumption; GENERATION; WASTES;

D O I：

10.1016/j.cej.2014.07.025

中图分类号：

X [环境科学、安全科学];

学科分类号：

08 ; 0830 ;

摘要：

The aim of this study was to investigate the feasibility of tetramethylammonium hydroxide (TMAH) production using the microbial electrolysis desalination and chemical-production cell (MEDCC). With 1.0 g/L acetate in the anode chamber and tetramethylammonium chloride solutions with different concentrations in the desalination chamber, TMAH could be efficiently produced in the cathode chamber of MEDCC. With an applied voltage of 1.0 V, the concentration of TMAH reached 0.087 M within 17.5 h, with current efficiency of 52-58%. The electrical energy consumed for the TMAH production using the MEDCC was 0.76 kWh/kg, which was only 5-12% of that for the electrolysis and electrodialysis process. With the high value of TMAH produced in a friendly environment with low energy consumption, the MEDCC should be a potentially valuable method for the chemical production in practice. (C) 2014 Elsevier B.V. All rights reserved.

引用

页码：157 / 162

页数：6

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