Molecular isomerization and fragmentation of polyatomic molecules controlled by inner-valence recollision-ionization

被引：0

作者：

Xie, X. ^{[1
]}

Doblhoff-Dier, K. ^{[2
]}

Roither, S. ^{[1
]}

Schoeffler, M. ^{[1
]}

Kartashov, D. ^{[1
]}

Xu, H. ^{[1
,3
]}

Rathje, T. ^{[4
]}

Paulus, G. G. ^{[4
]}

Baltuska, A. ^{[1
]}

Graefe, S.

Kitzler, M. ^{[1
]}

机构：

[1] Vienna Univ Technol, Photon Inst, A-1040 Vienna, Austria

[2] Vienna Univ Technol, Inst Theoret Phys, A-1040 Vienna, Austria

[3] Jilin Univ, State key Lab Integrated Optoelect, Changchun 130012, Peoples R China

[4] Univ Jena, Inst Opt & Quantum Elect, D-07743 Jena, Germany

来源：

XXVIII INTERNATIONAL CONFERENCE ON PHOTONIC, ELECTRONIC AND ATOMIC COLLISIONS (ICPEAC) | 2014年 / 488卷

关键词：

D O I：

10.1088/1742-6596/488/3/032012

中图分类号：

O59 [应用物理学];

学科分类号：

摘要：

Control over various fragmentation reactions of a series of polyatomic molecules (acetylene, ethylene 1,3-butadiene) by the optical waveform of intense few-cycle laser pulses is demonstrated experimentally. We show both experimentally and theoretically that the responsible mechanism is inelastic ionization from inner-valence molecular orbitals by recolliding electron wave packets.

引用

页数：1

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