Hydrophobic pillared square grids for selective removal of CO2 from simulated flue gas

被引：106

作者：

Elsaidi, Sameh K. ^{[1
,2
]}

Mohamed, Mona H. ^{[1
,3
]}

Schaef, Herbert T. ^{[2
]}

Kumar, Amrit ^{[4
]}

Lusi, Matteo ^{[4
]}

Pham, Tony ^{[3
]}

Forrest, Katherine A. ^{[3
]}

Space, Brian ^{[3
]}

Xu, Wenqian ^{[5
]}

Halder, Gregory J. ^{[5
]}

Liu, Jun ^{[2
]}

Zaworotko, Michael J. ^{[3
]}

Thallapally, Praveen K. ^{[2
]}

机构：

[1] Univ Alexandria, Fac Sci, Dept Chem, Alexandria 21321, Egypt

[2] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA

[3] Univ S Florida, Dept Chem, Tampa, FL 33620 USA

[4] Univ Limerick, Dept Chem & Environm Sci, Limerick, Ireland

[5] Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Argonne, IL 60439 USA

来源：

CHEMICAL COMMUNICATIONS | 2015年 / 51卷 / 85期

基金：

美国国家科学基金会;

关键词：

METAL-ORGANIC FRAMEWORKS; CARBON-DIOXIDE CAPTURE; POROUS MATERIALS; AQUEOUS AMMONIA; FUEL-CELLS; ADSORPTION; SEPARATION; STORAGE; DESIGN; BINDING;

D O I：

10.1039/c5cc06577a

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Capture of CO2 from flue gas is considered to be a feasible approach to mitigate the effects of anthropogenic emission of CO2. Herein we report that an isostructural family of metal organic materials (MOMs) of general formula [M(linker)(2)(pillar)], linker = pyrazine, pillar = hexaflourosilicate and M = Zn, Cu, Ni and Co exhibits highly selective removal of CO2 fromdry and wet simulated flue gas. Two members of the family, M = Ni and Co, SIFSIX-3-Ni and SIFSIX-3-Co, respectively, are reported for the first time and compared with the previously reported Zn and Cu analogs.

引用

页码：15530 / 15533

页数：4

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