Fabrication and Planar Cooling Performance of Flexible Bi0.5Sb1.5Te3/Epoxy Composite Thermoelectric Films

被引：10

作者：

Li Peng ^{[1
]}

Nie Xiao-Lei ^{[1
]}

Tian Ye ^{[1
]}

Fang Wen-Bing ^{[1
]}

Wei Ping ^{[1
]}

Zhu Wan-Ting ^{[1
]}

Sun Zhi-Gang ^{[1
]}

Zhang Qing-Jie ^{[1
]}

Zhao Wen-Yu ^{[1
]}

机构：

[1] Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Hubei, Peoples R China

来源：

JOURNAL OF INORGANIC MATERIALS | 2019年 / 34卷 / 06期

基金：

中国国家自然科学基金;

关键词：

flexible thermoelectric films; screen printing; Bi0.5Sb1.5Te3/epoxy composite films; electrical property; planar cooling field; POWER; GENERATORS; DEVICES; HEAT;

D O I：

10.15541/jim20180528

中图分类号：

TQ174 [陶瓷工业]; TB3 [工程材料学];

学科分类号：

0805 ; 080502 ;

摘要：

Flexible Bi0.5Sb1.5Te3/epoxy composite thermoelectric films were prepared on polyimide substrates by screen printing. Its electrical transport properties are enhanced by optimizing the content of Bi0.5Sb1.5Te3 powder. The highest power factor of the optimized Bi0.5Sb1.5Te3/epoxy films reached 1.12 mW.m(-1).K-2 at 300 K, increased by 33% as compared with previous value. The anti-bending test results show that resistance of the thick films remains unchanged when the bending radius is over 20 mm and slightly increases within 3000 bending cycles when the bending radius is 20 mm, implying that the as-prepared films have potential application in flexible TE devices. The flexible thermoelectric leg could establish a temperature difference from 4.2 degrees C to 7.8 degrees C under working current from 0.01 A to 0.05 A, showing potential application in planar cooling field.

引用

页码：679 / 684

页数：6

共 27 条

[1] Design of optimum plate-fin natural convective heat sinks
Bar-Cohen, A
Iyengar, M
Kraus, AD
[J]. JOURNAL OF ELECTRONIC PACKAGING, 2003, 125 (02) : 208 - 216
[2] Cooling, heating, generating power, and recovering waste heat with thermoelectric systems
Bell, Lon E.
[J]. SCIENCE, 2008, 321 (5895) : 1457 - 1461
[3] Flexible screen printed thermoelectric generator with enhanced processes and materials
Cao, Zhuo
Koukharenko, E.
Tudor, M. J.
Torah, R. N.
Beeby, S. P.
[J]. SENSORS AND ACTUATORS A-PHYSICAL, 2016, 238 : 196 - 206
[4] Nonequilibrium thermodynamic analysis of a thermoelectric device
Chen, JC
Yan, ZJ
Wu, LQ
[J]. ENERGY, 1997, 22 (10) : 979 - 985
[5] Heat transfer effect on the specific cooling load of refrigerators
Chen, LG
Wu, C
Sun, FR
[J]. APPLIED THERMAL ENGINEERING, 1996, 16 (12) : 989 - 997
[6] Chowdhury I, 2009, NAT NANOTECHNOL, V4, P235, DOI [10.1038/nnano.2008.417, 10.1038/NNANO.2008.417]
[7] Thermoelectric cooling and power generation
DiSalvo, FJ
[J]. SCIENCE, 1999, 285 (5428) : 703 - 706
[8] Fast preparation and high thermoelectric performance of the stable Bi0.5Sb1.5Te3 bulk materials for different synthesis pressures
Guo, Xin
Jia, Xiaopeng
Qin, Jieming
Sun, Hairui
Zhang, Yuewen
Sun, Bing
Liu, Binwu
Ma, Hongan
[J]. CHEMICAL PHYSICS LETTERS, 2014, 610 : 204 - 208
[9] High efficiency Bi2Te3-based materials and devices for thermoelectric power generation between 100 and 300 °C
Hao, Feng
Qiu, Pengfei
Tang, Yunshan
Bai, Shengqiang
Xing, Tong
Chu, Hsu-Shen
Zhang, Qihao
Lu, Ping
Zhang, Tiansong
Ren, Dudi
Chen, Jikun
Shi, Xun
Chen, Lidong
[J]. ENERGY & ENVIRONMENTAL SCIENCE, 2016, 9 (10) : 3120 - 3127
[10] Quantum dot superlattice thermoelectric materials and devices
Harman, TC
Taylor, PJ
Walsh, MP
LaForge, BE
[J]. SCIENCE, 2002, 297 (5590) : 2229 - 2232

← 1 2 3 →