Oxidative esterification of renewable furfural on gold-based catalysts: Which is the best support?

被引：69

作者：

Menegazzo, Federica ^{[1
,2
]}

Signoretto, Michela ^{[1
,2
]}

Pinna, Francesco ^{[1
,2
]}

Manzoli, Maela ^{[3
,4
]}

Aina, Valentina ^{[3
,4
]}

Cerrato, Giuseppina ^{[3
,4
]}

Boccuzzi, Flora ^{[3
,4
]}

机构：

[1] Ca Foscari Univ Venice, Dept Mol Sci & Nanosyst, I-30123 Venice, Italy

[2] RU Venice, Consortium INSTM, I-30123 Venice, Italy

[3] Univ Turin, Dept Chem, I-10125 Turin, Italy

[4] Univ Turin, NIS Ctr Excellence, I-10125 Turin, Italy

来源：

JOURNAL OF CATALYSIS | 2014年 / 309卷

关键词：

Gold catalyst; Furfural; Oxidation; Biomass; Effect of the support; QUANTITATIVE-DETERMINATION; AU/ZRO2; CATALYSTS; AEROBIC OXIDATION; ZIRCONIA; ACID; CO; SITES; CERIA;

D O I：

10.1016/j.jcat.2013.10.005

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

Gold-based catalysts over different supports were investigated in the oxidative esterification of furfural by employing an efficient and sustainable process. The catalytic performances follow the trend: Zirconia Au > Ceria-Au >> Titania Au. Zirconia came out to be the best support option to promote activity, selectivity and also stability. The chemical and morphological properties observed for zirconia-supported sample seem to fulfill a good compromise between high gold dispersion and the presence of suitable acid base properties, for good selectivity. Moreover, stability and recycling of the catalysts were also investigated. (C) 2013 Elsevier Inc. All rights reserved.

引用

页码：241 / 247

页数：7

共 50 条

[1] Gold-Based Nanoparticulate Catalysts for the Oxidative Esterification of 1,4-Butanediol to Dimethyl Succinate
Brett, Gemma L.
Miedziak, Peter J.
Knight, David W.
Taylor, Stuart H.
Hutchings, Graham J.
TOPICS IN CATALYSIS, 2014, 57 (6-9) : 723 - 729
[2] Gold-Based Nanoparticulate Catalysts for the Oxidative Esterification of 1,4-Butanediol to Dimethyl Succinate
Gemma L. Brett
Peter J. Miedziak
David W. Knight
Stuart H. Taylor
Graham J. Hutchings
Topics in Catalysis, 2014, 57 : 723 - 729
[3] O2 Adsorption and Oxidative Activity on Gold-Based Catalysts with and without a Ceria Support
Teng, Bo-Tao
Lang, Jia-Jian
Wen, Xiao-Dong
Zhang, Ce
Fan, Maohong
Harris, H. Gordon
JOURNAL OF PHYSICAL CHEMISTRY C, 2013, 117 (37): : 18986 - 18993
[4] Influence of Oxide Coating Layers on the Stability of Gold Catalysts for Furfural Oxidative Esterification to Methyl Furoate
Su, Juan
Zhan, Nannan
Tan, Yuan
Min, Xiangting
Xiao, Yan
Qiao, Botao
CATALYSTS, 2024, 14 (03)
[5] Biomass Derived Chemicals: Furfural Oxidative Esterification to Methyl-2-furoate over Gold Catalysts
Manzoli, Maela
Menegazzo, Federica
Signoretto, Michela
Marchese, Damiano
CATALYSTS, 2016, 6 (07):
[6] Gold-based catalysts for propylene epoxidation
Lu, Zheng
Piernavieja-Hermida, Mar
Wu, Zili
Lei, Yu
ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2016, 252
[7] Gold-Based Catalysts for Complete Formaldehyde Oxidation: Insights into the Role of Support Composition
Ilieva, Lyuba
Dimitrov, Dimitar
Kolentsova, Elitsa
Venezia, Anna Maria
Karashanova, Daniela
Avdeev, Georgi
Petrova, Petya
State, Razvan
Tabakova, Tatyana
CATALYSTS, 2022, 12 (07)
[8] Gold-based nanoparticle catalysts for catalytic applications
Dimitratos, Nikolaos
Hammond, Ceri
Hutchings, Graham J.
ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2014, 248
[9] Au/ZrO2: an efficient and reusable catalyst for the oxidative esterification of renewable furfural
Signoretto, M.
Menegazzo, F.
Contessotto, L.
Pinna, F.
Manzoli, M.
Boccuzzi, F.
APPLIED CATALYSIS B-ENVIRONMENTAL, 2013, 129 : 287 - 293
[10] Zeolite-encaged gold catalysts for the oxidative condensation of furfural
Li, Weijie
Gao, Mingyang
Qin, Bin
Deng, Xin
Li, Landong
FRONTIERS OF CHEMICAL SCIENCE AND ENGINEERING, 2024, 18 (08)

← 1 2 3 4 5 →