Methane Storage and Synthesis of HKUST-1 Prepared with Different Solvent

被引：0

作者：

Gong Xiaojie ^{[1
]}

Zhang Dan ^{[1
]}

Duan Linhai ^{[2
]}

Meng Xiuhong ^{[2
]}

Lin Wenjie ^{[3
]}

机构：

[1] Liaoning Shihua Univ, Sch Chem & Mat Sci, Fushun 113001, Peoples R China

[2] Guangdong Univ Petrochem Technol, Sch Chem Engn, Maoming 525000, Peoples R China

[3] Zhenghe Grp Co Ltd, Dongying 257000, Peoples R China

来源：

CHINA PETROLEUM PROCESSING & PETROCHEMICAL TECHNOLOGY | 2019年 / 21卷 / 02期

基金：

中国国家自然科学基金;

关键词：

HKUST-1; solubility; methane storage; METAL-ORGANIC FRAMEWORK; CATALYTIC PERFORMANCE; FACILE SYNTHESIS; GASEOUS TOLUENE; CO OXIDATION; MECHANISM; MOFS;

D O I：

暂无

中图分类号：

TE [石油、天然气工业]; TK [能源与动力工程];

学科分类号：

0807 ; 0820 ;

摘要：

The metal-organic framework HKUST-1 was prepared by different solvents. Several analytical tools such as scanning electron microscope (SEM), X-ray diffraction (XRD), N-2 adsorption-desorption have been used to characterize the as-synthesized samples. Meanwhile, the solubility of organic ligands in solvents and the CH4 adsorption capacity of samples were also detected. The results showed that HKUST-1 prepared with N,N-dimethylfonnamide (DMF) used as solvent exhibited excellent CH4 adsorption performance. Further studies have shown that the improved CH4 adsorption properties could be attributed to higher solubility of the ligand 1,3,5-benzenetricarboxylic acid in DMF and larger specific surface areas. This work can provide a novel sight for preparing highly efficient CH4 adsorbent materials by improving the solubility of ligand.

引用

页码：44 / 49

页数：6

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