The Jiangnan Orogen and Cathaysia Block constitute integral components in the geological framework of the South China Craton. However, the tectonic attributes of these two regions remain controversial. In this study we present LA-ICP-MS zircon U-Pb ages, Lu-Hf isotopes, and major and trace elements data from a suite of clastic rocks. Two hundred and forty seven zircon U-Pb ages obtained from the Neoproterozoic meta-sandstones in western Jiangnan Orogen define three major age populations: 2564-2395 Ma, 2068-1849 Ma and 963-730 Ma, corresponding to the early Paleoproterozoic crustal growth, amalgamation of the supercontinent Columbia and tectonics associated with Rodinia. Two hundred and forty three zircon U-Pb age data from Cambrian and Ordovician sandstones in the western Cathaysia yield five age populations: 2626-2392 Ma, 2050-1518 Ma, 1173-904 Ma, 857-708 Ma and 630-502 Ma, which can be correlated to the Neoarchean-early Paleoproterozoic continental growth, the tectono-thermal events associated with the Columbia supercontinent, the assembly and breakup of Rodinia, as well as the Pan-African event. The 630-502 Ma population correlates with the assembly of Gondwana supercontinent during late Neoproterozoic to early Paleozoic, although direct geological evidence for this event has not yet been reported from this region. These results suggest that the western Jiangnan belt and western Cathaysia Block have distinct crustal evolution histories albeit with close affinities. The REE geochemisty and Lu-Hf isotope data also indicate that the provenances of the Neoproterozoic and early Paleozoic detritus in western Jiangnan belt and western Cathaysia are mostly composed of reworked crustal materials. The metamorphic rims of zircon grains with core-rim structures yield ages of 912-891 Ma and 853-835 Ma, suggesting two phases of metamorphic events during Neoproterozoic in the source areas. These two events are likely associated with the tectonics related to the collision of Yangtze and Cathaysia blocks in the western and eastern segments, respectively. (C) 2015 Elsevier B.V. All rights reserved.