Wetting-drying cycles enhance the release and transport of autochthonous colloidal particles in Chinese loess

被引:19
|
作者
Zhou, Bo [1 ]
Wu, Yaoguo [1 ]
Chan, Jiangwei [1 ]
Wang, Sichang [1 ]
Qiao, Zixia [1 ]
Hu, Sihai [1 ]
机构
[1] Northwestern Polytech Univ, Dept Appl Chem, Xian 710072, Shaanxi, Peoples R China
来源
HUMAN AND ECOLOGICAL RISK ASSESSMENT | 2019年 / 25卷 / 1-2期
基金
中国国家自然科学基金;
关键词
wetting-drying cycles; autochthonous colloidal particles; release; transport; Chinese loess; GOLD MINING REGION; ANTHROPOGENIC POLLUTION; CONTAMINANT TRANSPORT; THEMATIC ISSUE; FRACTURED SOIL; MOBILIZATION; BEHAVIOR; GROUNDWATER; WATER; NANOPARTICLES;
D O I
10.1080/10807039.2019.1571402
中图分类号
X176 [生物多样性保护];
学科分类号
090705 ;
摘要
Soil columns packed by Chinese loess were tested under stimulated wetting-drying cycles. The results of leaching tests showed that ACPs concentration, although changed with initial peak concentration and secondary peak concentration, eventually tended to a stable level at about 6.0mgL(-1) within 48h. The results of wetting-drying cycle tests showed that the initial peak concentration, cumulative mass and mean size of ACPs increased with the length of drying period with the drying period. The initial peak concentration of ACPs after 90-d drying period was about nine times of that after 1d. In addition, the release and transport of ACPs increased with the wetting-drying cycles having the same drying duration. After ten wetting-drying cycles, the initial peak concentration of ACPs for 30-d drying period increased by 35.35% and that for 15d increased by 18.33%. The preliminary mechanisms to enhance the release and transport of ACPs include physical mechanisms of the air-water interface scouring, the shear stress of preferential flow and the collapsing pore walls by capillary pressure, and chemical mechanism of the salts dissolving of loess matrix. These findings are helpful to evaluate the risk of soil and groundwater pollution.
引用
收藏
页码:335 / 353
页数:19
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