Porous organic polymer with in situ generated palladium nanoparticles as a phase-transfer catalyst for Sonogashira cross-coupling reaction in water

被引：20
|
作者：
Dong, Ying [1 ]
Chen, Yun-Qi [1 ]
Jv, Jing-Jing [1 ]
Li, Yue [1 ]
Li, Wen-Han [1 ]
Dong, Yu-Bin [1 ]
机构：
[1] Shandong Normal Univ, Collaborat Innovat Ctr Functionalized Probes Chem, Coll Chem Chem Engn & Mat Sci, Key Lab Mol & Nano Probes,Minist Educ, Jinan 250014, Shandong, Peoples R China
来源：
RSC ADVANCES | 2019年 / 9卷 / 38期
基金：
中国国家自然科学基金;
关键词：
COPPER-FREE; EFFICIENT CATALYST; SUZUKI-MIYAURA; FRAMEWORK; CLAY; COMPOSITE; SUPPORT; COMPLEX;
D O I：
10.1039/c9ra04103f
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
A new Pd nanoparticle loaded and imidazolium-ionic liquid decorated organic polymer of Pd@PTC-POP was readily fabricated via a Pd(PPh3)(4) catalysed in situ one-pot Suzuki cross-coupling reaction between imidazolium attached dibromobenzene and 1,3,5-tri(4-pinacholatoborolanephenyl)benzene. Besides the high thermal and chemical stability, the obtained Pd@PTC-POP can be used as a highly active and reusable phase-transfer solid catalyst to promote the Sonogashira coupling reaction in water. The obtained results indicate that the Pd@PTC-POP herein could create a versatile family of solid phase transfer catalysts for promoting a broad scope of reactions carried out in water.
引用
收藏
页码：21671 / 21678
页数：8
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