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Are Multiphase Competition and Order by Disorder the Keys to Understanding Yb2Ti2O7?
被引:78
|作者:
Jaubert, L. D. C.
[1
]
Benton, Owen
[1
]
Rau, Jeffrey G.
[2
]
Oitmaa, J.
[3
]
Singh, R. R. P.
[4
]
Shannon, Nic
[1
]
Gingras, Michel J. P.
[2
,5
,6
]
机构:
[1] Okinawa Inst Sci & Technol Grad Univ, Onna Son, Okinawa 9040495, Japan
[2] Univ Waterloo, Dept Phys & Astron, Waterloo, ON N2L 3G1, Canada
[3] Univ New S Wales, Sch Phys, Sydney, NSW 2052, Australia
[4] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA
[5] Perimeter Inst Theoret Phys, Waterloo, ON N2L 2Y5, Canada
[6] Canadian Inst Adv Res, Toronto, ON M5G 1Z8, Canada
基金:
美国国家科学基金会;
加拿大自然科学与工程研究理事会;
关键词:
TRANSITION;
D O I:
10.1103/PhysRevLett.115.267208
中图分类号:
O4 [物理学];
学科分类号:
0702 ;
摘要:
If magnetic frustration is most commonly known for undermining long-range order, as famously illustrated by spin liquids, the ability of matter to develop new collective mechanisms in order to fight frustration is perhaps no less fascinating, providing an avenue for the exploration and discovery of unconventional behaviors. Here, we study a realistic minimal model where a number of such mechanisms converge, which, incidentally, pertain to the perplexing quantum spin ice candidate Yb2Sn2O7. Specifically, we explain how thermal and quantum fluctuations, optimized by order-by-disorder selection, conspire to expand the stability region of a degenerate continuous U(1) manifold against the classical splayed ferromagnetic ground state that is displayed by the sister compound Yb2Sn2O7. The resulting competition gives rise to multiple phase transitions, in striking similitude with recent experiments on Yb2Sn2O7 [Lhotel et al., Phys. Rev. B89, 224419 (2014)]. By combining a gamut of numerical techniques, we obtain compelling evidence that such multiphase competition is a natural engine for the substantial sample-to-sample variability observed in Yb2Sn2O7 and is the missing key to ultimately understand the intrinsic properties of this material. As a corollary, our work offers a pertinent illustration of the influence of chemical pressure in rare-earth pyrochlores.
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