Net transport due to noise-induced internal reciprocating motion

被引:9
|
作者
Makhnovskii, Yurii A. [1 ,2 ]
Rozenbaum, Viktor M. [1 ,3 ]
Yang, Dah-Yen [1 ]
Lin, Sheng Hsien [1 ,4 ]
机构
[1] Acad Sinica, Inst Atom & Mol Sci, Taipei 106, Taiwan
[2] Russian Acad Sci, AV Topchiev Petrochem Synth Inst, Moscow 119991, Russia
[3] Natl Acad Sci Ukraine, Chuiko Inst Surface Chem, UA-03164 Kiev, Ukraine
[4] Natl Chiao Tung Univ, Dept Appl Chem, Hsinchu 300, Taiwan
来源
JOURNAL OF CHEMICAL PHYSICS | 2009年 / 130卷 / 16期
关键词
BROWNIAN MOTORS; MOLECULAR MACHINES; SIMPLE-MODEL; RATCHET; PARTICLE; KINETICS; ENGINES; WALK;
D O I
10.1063/1.3116790
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We consider a system of two coupled Brownian particles fluctuating between two states. The fluctuations are produced by both equilibrium thermal and external nonthermal noise, the transition rates depending on the interparticle distance. An externally induced modulation of the transition rates acts on the internal degree of freedom (the interparticle distance) and generates reciprocating motion along this coordinate. The system moves unidirectionally due to rectification of the internal motion by asymmetric friction fluctuations and thus operates as a dimeric motor that converts input energy into net movement. The properties of the motor are primarily determined by the properties of the reciprocating engine, represented by the interparticle distance dynamics. Two main mechanisms are recognized by which the engine operates: energetic and informational. In the physically important cases where only one of the motion-inducing mechanisms is operative, exact solutions can be found for the model with linearly coupled particles. We focus on the informational mechanism, in which thermal noise is involved as a vital component and the reciprocating velocity exhibits a rich behavior as a function of the model parameters. An efficient rectification method for the reciprocating motion is also discussed. (C) 2009 American Institute of Physics. [DOI: 10.1063/1.3116790]
引用
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页数:10
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