Portable point-of-use photoelectrocatalytic device provides rapid water disinfection

被引:39
|
作者
Montenegro-Ayo, Renato [1 ,2 ]
Barrios, Ana C. [1 ]
Mondal, Indrayudh [3 ]
Bhagat, Kartik [1 ,4 ]
Carlos Morales-Gomero, Juan [2 ,5 ]
Abbaszadegan, Morteza [3 ]
Westerhoff, Paul [1 ]
Perreault, Francois [1 ]
Garcia-Segura, Sergi [1 ]
机构
[1] Arizona State Univ, Nanosyst Engn Res Ctr Nanotechnol Enabled Water T, Sch Sustainable Engn & Built Environm, Tempe, AZ 85287 USA
[2] Univ Lima, Fac Ingn & Arquitectura, Ave Javier Prado Este 4600, Santiago De Surco 1503, Peru
[3] Arizona State Univ, NSF Water & Environm Technol Ctr, Sch Sustainable Engn & Built Environm, Tempe, AZ 85287 USA
[4] Punjab Engn Coll, Dept Civil Engn, Sect 12, Chandigarh 160012, India
[5] Univ Nacl Ingn, Ctr Dev Adv Mat & Nanotechnol, Av Tupac Amaru 210, Lima 15333, Peru
基金
美国国家科学基金会;
关键词
Electrochemical advanced oxidation processes; Water treatment; TiO2 nanotubes photo-anodes; Translational technology; Escherichia coli; Legionella; ADVANCED OXIDATION PROCESSES; NATURAL ORGANIC-MATTER; SOLAR; PHOTOCATALYSIS; LEGIONELLA; INACTIVATION; DEGRADATION; NANOTUBES; ACCESS; IMPACT;
D O I
10.1016/j.scitotenv.2020.140044
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Portable water purification devices are needed to provide safe drinking water in rural communities, developing communities with low quality centralized water distribution, and military or recreational applications. Filtration, ultraviolet light, or chemical additives provide a spectrum of alternatives to remove pathogens from water. For the first time, we design, fabricate and demonstrate the performance of a small portable photoelectric point-of-use device, and document its performance on pathogen inactivation. The device utilizes a commercial teacup from which TiO2 nanotube photoanodes were produced in-situ and, with a small rechargeable battery powered 365 nm light emitting diode, was able to achieve 5-log inactivation of Escherichia coli in 10 s and 2.6-log of Legionella in 60 s of treatment in model water samples. Treatment of natural water achieved a 1-log bacteria inactivation after 30 s due to matrix effects. The electro-photocatalytic disinfection reactor in a kup (e-DRINK) can provide a feasible and affordable solution to ensure access to clean water. More broadly, this work demonstrates the potential for illumination to improve the efficiency of electrocatalytic surfaces. (C) 2020 Elsevier B.V. All rights reserved.
引用
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页数:8
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