Protein powder derived nitrogen-doped carbon supported atomically dispersed iron sites for selective oxidation of ethylbenzene

被引：12

作者：

Cheng, Yujie ^{[1
]}

Sun, Qingdi ^{[1
]}

Huang, Liyun ^{[1
]}

He, Qian ^{[1
]}

Zhang, Hao ^{[1
]}

Wang, Pengbo ^{[2
]}

Zhang, Ying ^{[3
]}

Shi, Shaolin ^{[2
]}

Zhang, Xingcong ^{[1
]}

Gan, Tao ^{[1
]}

He, Xiaohui ^{[1
,3
]}

Ji, Hongbing ^{[1
,2
,3
,4
]}

机构：

[1] Sun Yat Sen Univ, Sch Chem, Fine Chem Ind Res Inst, Guangzhou 510275, Guangdong, Peoples R China

[2] Guangxi Univ, Sch Chem & Chem Engn, Nanning 530004, Peoples R China

[3] Sun Yat Sen Univ, Huizhou Res Inst, Huizhou 516216, Peoples R China

[4] Guangdong Univ Petrochem Technol, Sch Chem Engn, Maoming 525000, Peoples R China

来源：

DALTON TRANSACTIONS | 2021年 / 50卷 / 34期

基金：

中国国家自然科学基金;

关键词：

POROUS CARBON; EFFICIENT; CATALYSTS; COBALT; NANOCATALYST; SULFOXIDES; ALCOHOLS; NITRIDE; SOLVENT; GREEN;

D O I：

10.1039/d1dt02001c

中图分类号：

O61 [无机化学];

学科分类号：

070301 ; 081704 ;

摘要：

Atomically dispersed Fe species embedded in the nitrogen-containing carbon supports (Fe-1/NC) are successfully synthesized using a ball milling approach, with commercial protein powder as the nitrogen source. The catalyst exhibits outstanding performance in the oxidation of aromatic compounds containing saturated C-H bonds into corresponding ketones under ambient conditions, which is superior to those of a nanoparticle catalyst (Fe-n/NC) and a metal-free catalyst (NC).

引用

页码：11711 / 11715

页数：6

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