Improved rate-based modeling of carbon dioxide absorption with aqueous monoethanolamine solution

被引：9

作者：

Moioli, Stefania ^{[1
]}

Pellegrini, Laura A. ^{[1
]}

Gamba, Simone ^{[1
]}

Li, Ben ^{[2
]}

机构：

[1] Dept Chem Mat & Chem Engn G Natta, I-20133 Milan, Italy

[2] Univ Sci & Technol, Sch Chem Engn, Anshan 114051, Peoples R China

来源：

FRONTIERS OF CHEMICAL SCIENCE AND ENGINEERING | 2014年 / 8卷 / 01期

关键词：

Absorption; carbon dioxide capture; rate-based model; monoethanolamine scrubbing; LOCAL COMPOSITION MODEL; EXCESS GIBBS ENERGY; CO2; CAPTURE; 30-MASS-PERCENT MONOETHANOLAMINE; EQUILIBRIUM-CONSTANTS; ELECTROLYTE SYSTEMS; GAS IMPURITIES; PLANT; MEA; THERMODYNAMICS;

D O I：

10.1007/s11705-014-1415-0

中图分类号：

TQ [化学工业];

学科分类号：

0817 ;

摘要：

This paper focuses on modeling and simulation of a post-combustion carbon dioxide capture in a coal-fired power plant by chemical absorption using monoethanolamine. The aim is to obtain a reliable tool for process simulation: a customized rate-based model has been developed and implemented in the ASPEN Plus(R) software, along with regressed parameters for the Electrolyte-NRTL model worked out in a previous research. The model is validated by comparison with experimental data of a pilot plant and can provide simulation results very close to experimental data.

引用

页码：123 / 131

页数：9

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Laura A. Pellegrini
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