Optical Stark Effects in J-Aggregate-Metal Hybrid Nanostructures Exhibiting a Strong Exciton-Surface-Plasmon-Polariton Interaction

被引：58
|
作者：
Vasa, P. [1 ,2 ]
Wang, W. [1 ]
Pomraenke, R. [1 ]
Maiuri, M. [3 ]
Manzoni, C. [3 ]
Cerullo, G. [3 ]
Lienau, C. [1 ]
机构：
[1] Carl von Ossietzky Univ Oldenburg, Inst Phys, D-26111 Oldenburg, Germany
[2] Indian Inst Technol, Dept Phys, Mumbai 400076, Maharashtra, India
[3] Politecn Milan, IFN CNR, Dipartimento Fis, I-20133 Milan, Italy
来源：
PHYSICAL REVIEW LETTERS | 2015年 / 114卷 / 03期
关键词：
SINGLE QUANTUM-DOT; SEMICONDUCTOR MICROCAVITIES; EMISSION;
D O I：
10.1103/PhysRevLett.114.036802
中图分类号：
O4 [物理学];
学科分类号：
0702 ;
摘要：
We report on the observation of optical Stark effects in J-aggregate-metal hybrid nanostructures exhibiting strong exciton-surface-plasmon-polariton coupling. For redshifted nonresonant excitation, pump-probe spectra show short-lived dispersive line shapes of the exciton-surface-plasmon-polariton coupled modes caused by a pump-induced Stark shift of the polariton resonances. For larger coupling strengths, the sign of the Stark shift is reversed by a transient reduction in normal mode splitting. Our studies demonstrate an approach to coherently control and largely enhance optical Stark effects in strongly coupled hybrid systems. This may be useful for applications in ultrafast all-optical switching.
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页数：6
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