CO2 Capture in Amine-Based Aqueous Solution: Role of the Gas-Solution Interface

被引：69

作者：

Lewis, Tanza ^{[1
]}

Faubel, Manfred ^{[2
]}

Winter, Bernd ^{[3
,4
]}

Hemminger, John C. ^{[1
]}

机构：

[1] Univ Calif Irvine, Dept Chem, Irvine, CA 92679 USA

[2] Max Planck Inst Dynam & Selbstorg, D-37037 Gottingen, Germany

[3] Helmholtz Zentrum Berlin Mat & Energie, D-12489 Berlin, Germany

[4] BESSY, D-12489 Berlin, Germany

来源：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2011年 / 50卷 / 43期

基金：

美国国家科学基金会;

关键词：

aqueous solution interfaces; carbon dioxide; photoelectron spectroscopy; CARBON-DIOXIDE; MONOETHANOLAMINE; KINETICS;

D O I：

10.1002/anie.201101250

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Interface matters! Photoelectron spectra of aqueous solutions of monoethanolamine (MEA) that had been treated with CO2 were used to determine the spatial distribution of MEA and the reaction products with respect to the solution interface (see picture). Neutral MEA shows a propensity for the solution surface, whereas protonated MEA and the reaction products prefer bulk solvation. © 2011 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

引用

页码：10178 / 10181

页数：4

共 50 条

[1] Tuning critical solution temperature for CO2 capture by aqueous solution of amine
Longeras, Olympe
Gautier, Arnaud
Ballerat-Busserolles, Karine
Andanson, Jean-Michel
JOURNAL OF MOLECULAR LIQUIDS, 2021, 343
[2] Tuning CO2 Capture at the Gas/Amine Solution Interface by Changing the Solvent Polarity
Gladich, Ivan
Abotaleb, Ahmed
Sinopoli, Alessandro
JOURNAL OF PHYSICAL CHEMISTRY B, 2020, 124 (45): : 10245 - 10256
[3] Research progress of aqueous amine solution for CO2 capture: A review
Meng, Fanzhi
Meng, Yuan
Ju, Tongyao
Han, Siyu
Lin, Li
Jiang, Jianguo
RENEWABLE & SUSTAINABLE ENERGY REVIEWS, 2022, 168
[4] Modeling aerosols in amine-based CO2 capture
Fulk, Steven M.
Rochelle, Gary T.
GHGT-11, 2013, 37 : 1706 - 1719
[5] Corrosivity of Amine-Based Absorbents for CO2 Capture
Gunasekaran, Prakashpathi
Veawab, Amornvadee
Aroonwilas, Adisorn
13TH INTERNATIONAL CONFERENCE ON GREENHOUSE GAS CONTROL TECHNOLOGIES, GHGT-13, 2017, 114 : 2047 - 2054
[6] Amine-based capture of CO2 for utilization and storage
Yamada, Hidetaka
POLYMER JOURNAL, 2021, 53 (01) : 93 - 102
[7] Amine-based adsorbents for CO2 capture from simulated flue gas
Xue, Guangxin
ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2016, 251
[8] Amine-based capture of CO2 for utilization and storage
Hidetaka Yamada
Polymer Journal, 2021, 53 : 93 - 102
[9] Desorption and mineralization of CO2 in amine-based solution by Ca(OH)2
Zhang, Weifeng
Li, Juan
Wang, Qiuhua
Qiu, Xuefei
INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL, 2020, 97
[10] Amine-based adsorbents for CO2 capture from simulated flue gas
Xue, Guangxin
ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2015, 250

← 1 2 3 4 5 →