The impact of local surface changes in Borneo on atmospheric composition at wider spatial scales: coastal processes, land-use change and air quality

被引：20

作者：

Pyle, J. A. ^{[1
]}

Warwick, N. J. ^{[1
]}

Harris, N. R. P. ^{[1
]}

Abas, Mohd Radzi ^{[11
]}

Archibald, A. T. ^{[1
]}

Ashfold, M. J. ^{[1
]}

Ashworth, K. ^{[2
]}

Barkley, Michael P. ^{[3
,4
]}

Carver, G. D. ^{[1
]}

Chance, K. ^{[5
]}

Dorsey, J. R. ^{[6
]}

Fowler, D. ^{[7
]}

Gonzi, S. ^{[3
]}

Gostlow, B. ^{[1
]}

Hewitt, C. N. ^{[2
]}

Kurosu, T. P. ^{[5
]}

Lee, J. D. ^{[8
]}

Langford, S. B. ^{[2
]}

Mills, G. ^{[13
]}

Moller, S. ^{[8
]}

MacKenzie, A. R. ^{[2
]}

Manning, A. J. ^{[9
]}

Misztal, P. ^{[7
,10
]}

Nadzir, Mohd Shahrul Mohd ^{[11
]}

Nemitz, E. ^{[7
]}

Newton, H. M. ^{[13
]}

O'Brien, L. M. ^{[1
]}

Ong, Simon ^{[14
]}

Oram, D. ^{[13
]}

Palmer, P. I. ^{[3
]}

Peng, Leong Kok ^{[15
]}

Phang, Siew Moi ^{[11
]}

Pike, R. ^{[1
]}

Pugh, T. A. M. ^{[2
]}

Rahman, Noorsaadah Abdul ^{[12
]}

Robinson, A. D. ^{[1
]}

Sentian, J. ^{[16
]}

Abu Samah, Azizan ^{[11
]}

Skiba, U. ^{[7
]}

Ung, Huan Eng ^{[14
]}

Yong, Sei Eng ^{[15
]}

Young, P. J. ^{[1
,17
,18
]}

机构：

[1] Univ Cambridge, Dept Chem, Cambridge CB2 1EW, England

[2] Univ Lancaster, Lancaster Environm Ctr, Lancaster LA1 4YQ, England

[3] Univ Edinburgh, Sch Geosci, Edinburgh EH9 3JW, Midlothian, Scotland

[4] Univ Leicester, Dept Phys & Astron, Leicester LE1 7RH, Leics, England

[5] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA

[6] Univ Manchester, Sch Earth Atmospher & Environm Sci, Manchester M13 3PL, Lancs, England

[7] Ctr Ecol & Hydrol, Penicuik EH26 0QB, Midlothian, Scotland

[8] Univ York, Dept Chem, York YO10 5DD, N Yorkshire, England

[9] Met Off, Exeter, Devon, England

[10] Univ Edinburgh, Dept Chem, Edinburgh EH8 9YL, Midlothian, Scotland

[11] Univ Malaya, Inst Ocean & Earth Sci, Kuala Lumpur 50603, Malaysia

[12] Univ Malaya, Dept Chem, Kuala Lumpur 50603, Malaysia

[13] Univ E Anglia, Sch Environm Sci, Norwich NR4 7TJ, Norfolk, England

[14] Global Satria Life Sci Lab, Tawau 91000, Sabah, Malaysia

[15] Ketua Stesen GAW Lembah Danum, Malaysian Meteorol Dept, Tawau 91011, Sabah, Malaysia

[16] Univ Malaysia Sabah, Sch Sci & Technol, Kota Kinabalu, Malaysia

[17] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA

[18] NOAA, Earth Syst Res Lab, Boulder, CO USA

来源：

PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY B-BIOLOGICAL SCIENCES | 2011年 / 366卷 / 1582期

关键词：

tropospheric ozone; biogenic organic compounds; rainforest; isoprene; atmospheric modelling; TROPICAL RAIN-FOREST; MARINE BOUNDARY-LAYER; TERRESTRIAL ISOPRENE EMISSIONS; VOLATILE ORGANIC-COMPOUNDS; OZONE DESTRUCTION; ATLANTIC-OCEAN; BOX MODEL; EAST; TROPOSPHERE; GASES;

D O I：

10.1098/rstb.2011.0060

中图分类号：

Q [生物科学];

学科分类号：

07 ; 0710 ; 09 ;

摘要：

We present results from the OP3 campaign in Sabah during 2008 that allowus to study the impact of local emission changes over Borneo on atmospheric composition at the regional and wider scale. OP3 constituent data provide an important constraint on model performance. Treatment of boundary layer processes is highlighted as an important area of model uncertainty. Model studies of land-use change confirm earlier work, indicating that further changes to intensive oil palm agriculture in South East Asia, and the tropics in general, could have important impacts on air quality, with the biggest factor being the concomitant changes in NOx emissions. With the model scenarios used here, local increases in ozone of around 50 per cent could occur. We also report measurements of short-lived brominated compounds around Sabah suggesting that oceanic (and, especially, coastal) emission sources dominate locally. The concentration of bromine in short-lived halocarbons measured at the surface during OP3 amounted to about 7 ppt, setting an upper limit on the amount of these species that can reach the lower stratosphere.

引用

页码：3210 / 3224

页数：15

共 17 条

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