Magnetic-Field-Tunable Intensity Transfer from Optically Active Phonons to Crystal-Field Excitations in the Reflection Spectra of the PrFe3(BO3)4 Antiferromagnet
intensities of coupled electron-phonon modes;
PrFe3(BO3)(4);
theory of intensity transfer;
MAGNETOELECTRIC PROPERTIES;
EARTH;
ION;
D O I:
10.3390/cryst12030392
中图分类号:
O7 [晶体学];
学科分类号:
0702 ;
070205 ;
0703 ;
080501 ;
摘要:
We analyze the field-dependent intensities of the coupled electron-phonon modes observed in the low-temperature far-infrared (terahertz) reflection spectra of PrFe3(BO3)(4) and develop a theory based on the Green's function approach. An excellent agreement between the experimental and theoretical data is achieved. The developed theory of the intensity transfer from phonons to quasi-electronic excitations can be applied to the electron-phonon modes in other compounds, in particular, in magnetodielectric materials, where it can be used to analyze the magnetodielectric response.
机构:
Institute of Spectroscopy, Russian Academy of Sciences, Troitsk
Moscow Institute of Physics and Technology, State University, DolgoprudnyInstitute of Spectroscopy, Russian Academy of Sciences, Troitsk
Stanislavchuk T.N.
Popova M.N.
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机构:
Institute of Spectroscopy, Russian Academy of Sciences, TroitskInstitute of Spectroscopy, Russian Academy of Sciences, Troitsk
Popova M.N.
Malkin B.Z.
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机构:
Kazan State UniversityInstitute of Spectroscopy, Russian Academy of Sciences, Troitsk
Malkin B.Z.
Bezmaternykh L.N.
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机构:
Kirensky Institute of Physics, Siberian Branch, Russian Academy of SciencesInstitute of Spectroscopy, Russian Academy of Sciences, Troitsk