Atmospheric carbonyl compounds in Chinese background area: A remote mountain of the Qinghai-Tibetan Plateau

被引:30
|
作者
Mu, Yujing [1 ]
Pang, Xiaobing
Quan, Jiannong
Zhang, Xiaoshan
机构
[1] Chinese Acad Sci, Res Ctr Eco Environm Sci, Dept Atmospher Chem, Beijing, Peoples R China
[2] Nankai Univ, Coll Environm Sci & Engn, Tianjin 300071, Peoples R China
关键词
OBSERVATORY PHOTOCHEMISTRY EXPERIMENT; MAUNA-LOA; PEROXYACETYL NITRATE; OZONE; FORMALDEHYDE; EMISSIONS; ISOPRENE; WALIGUAN; HYDROCARBONS; TROPOSPHERE;
D O I
10.1029/2006JD008211
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
[1] The ambient concentrations of carbonyl compounds were measured in Waliguan (WLG) Observatory at the east edge of Qinghai-Tibetan in August - September and December, 2005. The average concentrations of formaldehyde, acetaldehyde, acetone, and 2-butenal were 4.16 +/- 1.89, 4.25 +/- 3.32, 2.02 +/- 0.86, and 1.93 +/- 1.58 ppbv (n = 42), respectively, in August - September and 1.48 +/- 0.42, 3.91 +/- 0.81, 1.88 +/- 0.69, and 0.69 +/- 0.16 ppbv (n = 12), respectively, in December. Biomass used as fuel for cooking by local residents was considered as the dominant source for 2-butenal. Photooxidation of VOC (especially biogenic emission of isoprene) was one source for formaldehyde and methyl vinyl ketone in August - September. Animal excrement was probably an additional source for formaldehyde and acetone. Back trajectory analysis indicated that long-distance transportation from polluted air might be one important source for formaldehyde, acetone, and acetaldehyde in WLG.
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页数:10
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