Supported Au catalysts for propene total oxidation: Study of support morphology and gold particle size effects

被引：30
|
作者：
Ousmane, M. [2 ,3 ,4 ]
Liotta, L. F. [1 ]
Pantaleo, G. [1 ]
Venezia, A. M. [1 ]
Di Carlo, G. [5 ]
Aouine, M. [2 ,3 ,4 ]
Retailleau, L. [2 ,3 ,4 ]
Giroir-Fendler, A. [2 ,3 ,4 ]
机构：
[1] CNR, ISMN, I-90146 Palermo, Italy
[2] Univ Lyon, F-69003 Lyon, France
[3] Univ Lyon 1, F-69622 Villeurbanne, France
[4] CNRS, IRCELYON, UMR 5256, F-69622 Villeurbanne, France
[5] CNR, ISMN, I-00015 Monterotondo, Italy
来源：
CATALYSIS TODAY | 2011年 / 176卷 / 01期
关键词：
Au; TiO2; ZnO; Al2O3; Propene oxidation; Au particle size; Metal-support interaction; Support morphology; CO OXIDATION; AMBIENT-TEMPERATURE; METAL OXIDES; OXYGEN; PERFORMANCE; 2-PROPANOL; MECHANISM; AU/AL2O3; AU/TIO2; AU/ZNO;
D O I：
10.1016/j.cattod.2011.07.009
中图分类号：
O69 [应用化学];
学科分类号：
081704 ;
摘要：
In this work gold nanoparticles supported over three different metal oxides, TiO2, ZnO and Al2O3 were characterized by BET surface area and pore size distribution, XRD, XPS and TEM techniques and their catalytic performances were evaluated in the total oxidation of propene, chosen as model VOC molecule. Attention was focused on the evaluation of the catalytic activity by performing three consecutive catalytic runs. Characterizations by XPS and TEM were carried out on the spent catalysts after propene oxidation tests. The results were discussed in terms of relationship between morphological, structural, electronic and catalytic properties as a function of the nature of the support. (C) 2011 Elsevier B.V. All rights reserved.
引用
收藏
页码：7 / 13
页数：7
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