Two-dimensional metal-organic frameworks with high oxidation states for efficient electrocatalytic urea oxidation

被引：367
|
作者：
Zhu, Dongdong [1 ]
Guo, Chunxian [1 ]
Liu, Jinlong [1 ]
Wang, Liang [2 ]
Dub, Yi [2 ]
Qiao, Shi-Zhang [1 ]
机构：
[1] Univ Adelaide, Sch Chem Engn, Adelaide, SA 5005, Australia
[2] Univ Wollongong, ISEM, Wollongong, NSW 2525, Australia
来源：
CHEMICAL COMMUNICATIONS | 2017年 / 53卷 / 79期
基金：
中国国家自然科学基金; 澳大利亚研究理事会;
关键词：
OXYGEN-EVOLUTION; ELECTROCHEMICAL EVOLUTION; ELECTROOXIDATION; NANOSHEETS; CATALYSTS; OXIDE;
D O I：
10.1039/c7cc06378d
中图分类号：
O6 [化学];
学科分类号：
0703 ;
摘要：
A two-dimensional metal-organic framework (MOF) comprising nickel species and an organic ligand of benzenedicarboxylic acid is fabricated and explored as an electrocatalyst for urea oxidation reaction (UOR). The excellent UOR performance is found to be partially due to the high active site density of the two-dimensional MOF, and largely because of the high oxidation state of the nickel species.
引用
收藏
页码：10906 / 10909
页数：4
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