Dielectric and magnetic anomalies and spin frustration in hexagonal RMnO3 (R = Y, Yb, and Lu) -: art. no. 104419

被引:418
作者
Katsufuji, T [1 ]
Mori, S
Masaki, M
Moritomo, Y
Yamamoto, N
Takagi, H
机构
[1] Univ Tokyo, Dept Adv Mat Sci, Tokyo 1138656, Japan
[2] Univ Tokyo, Dept Appl Chem, Tokyo 1138656, Japan
[3] Tokyo Inst Technol, Dept Phys, Tokyo 1528551, Japan
[4] Nagoya Univ, CIRSE, Nagoya, Aichi 4648601, Japan
[5] Nagoya Univ, Dept Crystalline Mat Sci, Nagoya, Aichi 4648601, Japan
关键词
D O I
10.1103/PhysRevB.64.104419
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Single crystals of hexagonal RMnO3 (R = Y, Yb, and Lu), where Mn ions form the triangular lattice, were investigated, focusing on their dielectric/magnetic anomalies as well as geometrical spin frustration. It is found that the ratio of a Weiss temperature to T-N is similar to 10 in RMnO3, indicating the dominant role of strong geometrical frustration. The effect of geometrical frustration also appears in specific heat, which shows a presence of a substantial amount of residual magnetic contribution below T-N, indicating that a part of the spins are still fluctuating at T much less thanT(N). It is also found that the dielectric anomaly at T-N is strongly anisotropic, suggesting a unique correlation between magnetism and dielectric properties in these compounds.
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共 22 条
[1]   STRUCTURE MAGNETIQUE DE MNYO3 [J].
BERTAUT, EF ;
MERCIER, M .
PHYSICS LETTERS, 1963, 5 (01) :27-29
[2]   Magnetic structure and spin reorientation transition in ScMnO3 [J].
Bieringer, M ;
Greedan, JE .
JOURNAL OF SOLID STATE CHEMISTRY, 1999, 143 (01) :132-139
[3]   MAGNETIC-SUSCEPTIBILITIES OF THE FRUSTRATED TRIANGULAR LATTICE ANTI-FERROMAGNETS CSVCL3 AND VX2 (X=CL, BR AND I) - APPEARANCE OF MAGNETIC LIQUID IN THE ORDERED STATE [J].
HIRAKAWA, K ;
IKEDA, H ;
KADOWAKI, H ;
UBUKOSHI, K .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 1983, 52 (08) :2882-2887
[4]   Coupling between the ferroelectric and antiferromagnetic orders in YMnO3 [J].
Huang, ZJ ;
Cao, Y ;
Sun, YY ;
Xue, YY ;
Chu, CW .
PHYSICAL REVIEW B, 1997, 56 (05) :2623-2626
[5]  
ISMAILZA IG, 1965, FIZ TVERD TELA+, V7, P236
[6]   Dielectric anomalies at magnetic transitions of hexagonal rare earth manganese oxides RMnO3 [J].
Iwata, N ;
Kohn, K .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 1998, 67 (09) :3318-3319
[7]   BIREFRINGENCE STUDY ON STRUCTURAL AND MAGNETIC PHASE-TRANSITIONS OF RBMNBR3 [J].
KATO, T ;
IIO, K ;
HOSHINO, T ;
MITSUI, T ;
TANAKA, H .
JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN, 1992, 61 (01) :275-285
[9]   Ferroelectricity of YMnO3 thin films prepared via solution [J].
Kitahata, H ;
Tadanaga, K ;
Minami, T ;
Fujimura, N ;
Ito, T .
APPLIED PHYSICS LETTERS, 1999, 75 (05) :719-721
[10]   A NOTE ON THE MAGNETIC STRUCTURES OF RARE EARTH MANGANESE OXIDES [J].
KOEHLER, WC ;
YAKEL, HL ;
WOLLAN, EO ;
CABLE, JW .
PHYSICS LETTERS, 1964, 9 (02) :93-95