Phonon drag thermal Hall effect in metallic strontium titanate

被引:11
|
作者
Jiang, Shan [1 ]
Li, Xiaokang [1 ]
Fauque, Benoit [2 ]
Behnia, Kamran [1 ]
机构
[1] PSL Univ, Sorbonne Univ, Lab Phys & Etud Mat, Ecole Super Phys & Chim Ind ESPCI Paris CNRS, F-75005 Paris, France
[2] Paris Sci & Lettres PSL Univ, Coll France, Jeunes Equipes Inst Phys JEIP, Unite Serv & Rech USR 3573 CNRS, F-75231 Paris 05, France
关键词
quantum paralectric; thermal Hall effect; dilute metal; Hall angle; phonon drag; PHASE; CONDUCTIVITY; TRANSITION;
D O I
10.1073/pnas.2201975119
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
SrTiO3, a quantum paralectric, displays a detectable phonon thermalHall effect (THE). Here, we show that the amplitude of the THE is extremely sensitive to stoichiometry. It drastically decreases upon substitution of a tiny fraction of Sr atoms with Ca, which stabilizes the ferroelectric order. It drastically increases by an even lower density of oxygen vacancies, which turn the system to a dilute metal. The enhancement in the metallic state exceeds by far the sum of the electronic and the phononic contributions. We explain this observation as an outcome of three features: 1) Heat is mostly transported by phonons; 2) the electronic Hall angle is extremely large; and 3) there is substantial momentum exchange between electrons and phonons. Starting from Herring's picture of phonon drag, we arrive to a quantitative account of the enhanced THE. Thus, phonon drag, hitherto detected as an amplifier of thermoelectric coefficients, can generate a purely thermal transverse response in a dilute metal with a large Hall angle. Our results reveal a hitherto-unknown consequence of momentum-conserving collisions between electrons and phonons.
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页数:7
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