Pt nanoparticles decorated rose-like Bi2O2CO3 configurations for efficient photocatalytic removal of water organic pollutants

被引:9
|
作者
Chen, Huijuan [1 ]
Zhou, Zhongfu [2 ,3 ,4 ]
Greaves, G. Neville [4 ,5 ,6 ]
Nigar, Salma [1 ]
Cao, Huaqiang [7 ]
Zhao, Tingkai [8 ]
Lu, Xionggang [2 ]
机构
[1] Shanghai Univ, Sch Mat Sci & Engn, Shanghai 200444, Peoples R China
[2] Shanghai Univ, State Key Lab Adv Special Steel, Shanghai 200072, Peoples R China
[3] Shanghai Univ, Key Lab Mat Microstruct, Shanghai 200444, Peoples R China
[4] Aberystwyth Univ, Dept Phys, Aberystwyth SY23 3BZ, Dyfed, Wales
[5] Wuhan Univ Technol, State Key Lab Silicate Mat Architectures, Wuhan 430070, Hubei, Peoples R China
[6] Univ Cambridge, Dept Mat Sci & Met, Charles Babbage Rd, Cambridge CB2 3QZ, England
[7] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China
[8] Northwestern Polytech Univ, Sch Mat Sci & Engn, State Key Lab Solidificat Proc, Xian 710072, Shaanxi, Peoples R China
来源
RSC ADVANCES | 2018年 / 8卷 / 02期
关键词
LIGHT; MICROSPHERES; DEGRADATION; PERFORMANCE; COMPOSITE; AU; OXIDATION; CATALYST; UV;
D O I
10.1039/c7ra12236e
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Pt nanoparticles decorated with rose-like Bi2O2CO3 configurations were synthesized via a simple photoreduction method at room temperature. The structure, morphology, optical and electronic properties, and photocatalytic performance of the as-prepared materials were characterized. Compared to pure Bi2O2CO3, the Pt/Bi2O2CO3 photocatalysts show better performance in decomposing RhB, BPA and OTC under visible light (lambda > 420 nm). The enhanced photocatalytic activity of Pt/Bi2O2CO3 could be attributed to the modification in light absorption (lambda > 420 nm) charge migration and the separation of photo-generated electrons (e(-)) and holes (h(+)). Free radical trapping experiments demonstrated that the main active species of the catalytic reaction are different in decomposing RhB and BPA.
引用
收藏
页码:914 / 920
页数:7
相关论文
共 50 条
  • [1] Preparation of rose-like Bi2O2CO3 photocatalyst with enhanced performance for photocatalytic degradation of mineral flotation wastewater
    Huang, Yong
    He, Linxin
    Huang, Pan
    Ye, Yuling
    Xing, Bo
    Guo, Dejin
    Wu, Wenying
    Zeng, Ying
    INORGANIC CHEMISTRY COMMUNICATIONS, 2023, 158
  • [2] A facile way for one-pot synthesis of porous rose-like β-Bi2O3/Bi2O2CO3 with enhanced photocatalytic activity for BPA photodegradation
    Sipin Zhu
    Xiaoqi Wen
    Jin Zeng
    Chunying Wang
    Xianping Luo
    Journal of Materials Science, 2022, 57 : 19356 - 19370
  • [3] A facile way for one-pot synthesis of porous rose-like β-Bi2O3/Bi2O2CO3 with enhanced photocatalytic activity for BPA photodegradation
    Zhu, Sipin
    Wen, Xiaoqi
    Zeng, Jin
    Wang, Chunying
    Luo, Xianping
    JOURNAL OF MATERIALS SCIENCE, 2022, 57 (41) : 19356 - 19370
  • [4] Rose-like I-doped Bi2O2CO3 microspheres with enhanced visible light response: DFT calculation, synthesis and photocatalytic performance
    Zai, Jiantao
    Cao, Fenglei
    Liang, Na
    Yu, Ke
    Tian, Yuan
    Sun, Huai
    Qian, Xuefeng
    JOURNAL OF HAZARDOUS MATERIALS, 2017, 321 : 464 - 472
  • [5] Removal of MCs by Bi2O2CO3: adsorption and the potential of photocatalytic degradation
    Wang, Yujiao
    Cao, Yanqiu
    Li, Hongmei
    Gong, Aijun
    Han, Jintao
    Qian, Zhen
    Chao, Wenran
    ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH, 2018, 25 (12) : 11867 - 11874
  • [6] Removal of MCs by Bi2O2CO3: adsorption and the potential of photocatalytic degradation
    Yujiao Wang
    Yanqiu Cao
    Hongmei Li
    Aijun Gong
    Jintao Han
    Zhen Qian
    Wenran Chao
    Environmental Science and Pollution Research, 2018, 25 : 11867 - 11874
  • [7] Fabrication of β-phase AgI and Bi2O3 co-decorated Bi2O2CO3 heterojunctions with enhanced photocatalytic performance
    Wang, Qi
    Zhang, Chenlu
    Wu, Hong
    Gao, Qiaoyuan
    Duan, Ran
    Chen, Chuncheng
    JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2019, 547 : 1 - 13
  • [8] Rod-like Bi4O7 decorated Bi2O2CO3 plates: Facile synthesis, promoted charge separation, and highly efficient photocatalytic degradation of organic contaminants
    Sun, Meng
    Yan, Tao
    Zhang, Yaru
    He, Yunhui
    Shao, Yu
    Wei, Qin
    Du, Bin
    JOURNAL OF COLLOID AND INTERFACE SCIENCE, 2018, 514 : 240 - 249
  • [9] Cu2O NPs/Bi2O2CO3 flower-like complex photocatalysts with enhanced visible light photocatalytic degradation of organic pollutants
    Lin, Shuanglong
    Cui, Wenquan
    Li, Xingang
    Sui, Hong
    Zhang, Zisheng
    CATALYSIS TODAY, 2017, 297 : 237 - 245
  • [10] Enhanced photocatalytic degradation for organic pollutants by a novel m-Bi2O4/Bi2O2CO3 photocatalyst under visible light
    Wang, Junxiu
    Chen, Kuan
    Shen, Yi
    Wang, Xi
    Guo, Yongfu
    Zhou, Xiaoji
    Bai, Renbi
    RESEARCH ON CHEMICAL INTERMEDIATES, 2018, 44 (05) : 3061 - 3079