A generalized reduced fluid dynamic model for flow fields and electrodes in redox flow batteries

被引:6
|
作者
Cheng, Ziqiang [1 ]
Tenny, Kevin [2 ,3 ]
Pizzolato, Alberto [1 ]
Forner-Cuenca, Antoni [4 ]
Verda, Vittorio [1 ]
Chiang, Yet-Ming [2 ,5 ]
Brushett, Fikile [2 ,3 ]
Behrou, Reza [6 ]
机构
[1] Politecn Torino, Dept Energy, Turin, Italy
[2] MIT, Joint Ctr Energy Storage Res, 77 Massachusetts Ave, Cambridge, MA 02139 USA
[3] MIT, Dept Chem Engn, Cambridge, MA 02139 USA
[4] Eindhoven Univ Technol, Dept Chem Engn & Chem, Eindhoven, Netherlands
[5] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA
[6] Univ Calif San Diego, Dept Mech & Aerosp Engn, La Jolla, CA 92093 USA
基金
荷兰研究理事会; 美国国家科学基金会;
关键词
depth-averaging; electrode; flow field; fluid dynamics; numerical modeling; redox flow batteries; 3-DIMENSIONAL MODEL; PORE-SCALE; PERFORMANCE; DESIGN; CHANNEL; DEPTH; TRANSPORT; GEOMETRY; PROGRESS;
D O I
10.1002/aic.17540
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
High-dimensional models typically require a large computational overhead for multiphysics applications, which hamper their use for broad-sweeping domain interrogation. Herein, we develop a modeling framework to capture the through-plane fluid dynamic response of electrodes and flow fields in a redox flow cell, generating a computationally inexpensive two-dimensional (2D) model. We leverage a depth-averaging approach that also accounts for variations in out-of-plane fluid motion and departures from Darcy's law that arise from averaging across three-dimensions (3D). Our resulting depth-averaged 2D model successfully predicts the fluid dynamic response of arbitrary in-plane flow field geometries, with discrepancies of <5% for both maximum velocity and pressure drop. This corresponds to reduced computational expense, as compared to 3D representations (<1% of duration and 10% of RAM usage), providing a platform to screen and optimize a diverse set of cell geometries.
引用
收藏
页数:14
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