A new perylene diimide-based fluorescent chemosensor for selective detection of ATP in aqueous solution

被引：44
|
作者：
Yan, Liwei [1 ,2 ]
Ye, Zhongbin [1 ,2 ]
Peng, Chunxiang [2 ]
Zhang, Shihong [2 ]
机构：
[1] SW Petr Univ, State Key Lab Oil & Gas Reservoir Geol & Exploita, Chengdu 610500, Sichuan, Peoples R China
[2] SW Petr Univ, Sch Chem & Chem Engn, Chengdu 610500, Sichuan, Peoples R China
来源：
TETRAHEDRON | 2012年 / 68卷 / 12期
基金：
中国国家自然科学基金;
关键词：
Fluorescent; Chemosensor; ATP; Detection; Perylene diimide (PDI); SENSOR; PYROPHOSPHATE; RECOGNITION; CONJUGATE; DESIGN;
D O I：
10.1016/j.tet.2012.01.028
中图分类号：
O62 [有机化学];
学科分类号：
070303 ; 081704 ;
摘要：
A new perylene diimide (PDI) ligand (1) functionalized with a Zn2+-dipicolylethylenediamine (Zn2+-DPEN) moiety was synthesized and first used as a fluorometric chemosensor to specifically detect the presence of ATP over other phosphate anions in aqueous solution. The solution of 1 upon addition of ATP displayed a remarkable absorption decrease compared with other anions, indicating the selectivity of 1 to ATP. Moreover, among these anions investigated, only ATP showed a considerable enhancement of fluorescent intensity of 1. The fluorescence molar ratio plot combined with the ESI-TOF mass measurement determined that binding stoichiometry between 1 and ATP is 1:1. (C) 2012 Elsevier Ltd. All rights reserved.
引用
收藏
页码：2725 / 2727
页数：3
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