Modelling Deposition and Erosion rates with RadioNuclides (MODERN) - Part 2: A comparison of different models to convert 239+240Pu inventories into soil redistribution rates at unploughed sites

被引:24
|
作者
Arata, Laura [1 ]
Alewell, Christine [1 ]
Frenkel, Elena [2 ]
A'Campo-Neuen, Annette [3 ]
Iurian, Andra-Rada [4 ,5 ]
Ketterer, Michael E. [6 ]
Mabit, Lionel [7 ]
Meusburger, Katrin [1 ]
机构
[1] Univ Basel, Dept Environm Sci, Environm Geosci, CH-4003 Basel, Switzerland
[2] Univ Strasbourg, IRMA, Strasbourg, France
[3] Univ Basel, Dept Math & Comp Sci, CH-4003 Basel, Switzerland
[4] Univ Babes Bolyai, Fac Environm Sci & Engn, Cluj Napoca, Romania
[5] Univ Plymouth, Consolidated Radioisotope Facil, Plymouth, Devon, England
[6] Metropolitan State Univ Denver, Dept Chem, Denver, CO USA
[7] FAO IAEA Agr & Biotechnol Lab, Soil & Water Management & Crop Nutr Lab, Seibersdorf, Austria
基金
瑞士国家科学基金会;
关键词
Soil erosion; Plutonium; Inventory method; Diffusion and migration model; Profile distribution model; Proportional model; CESIUM-137; MEASUREMENTS; CS-137; PLUTONIUM; MIGRATION; TRACERS;
D O I
10.1016/j.jenvrad.2016.05.009
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Sheeterosion is one of the major threats to alpine soils. To quantify its role and impact in the degradation processes of alpine grasslands, the application of Fallout Radionuclides (FRN) showed very promising results. The specific characteristics of plutonium 239 + 240 (Pu239+240), such as the homogeneous fallout distribution, the long half-life and the cost and time effective measurements make this tracer application for investigating soil degradation in Alpine "grasslands more suitable than any other FRN (e.g. Cs-137). However, the conversion of Pu239+240 inventories into soil erosion rates remains a challenge. Currently available conversion models have been developed mainly for Cs-137 with later adaptation to other FRN (e.g. Excess Pb-210, and Be-7), each model being defined for specific land use (ploughed and/or unploughed) and processes (erosion or deposition). As such, they may fail in describing correctly the distribution of Pu isotopes in the soil. A new conversion model, MODERN, with an adaptable algorithm to estimate erosion and deposition rates from any FRN inventory changes was recently proposed (Arata et al., 2016). In this complementary contribution, the authors compare the application of MODERN to other available conversion models. The results show a good agreement between soil redistribution rates obtained from MODERN and from the models currently used by the FRN scientific community (i.e. the Inventory Method). (C) 2016 The Authors. Published by Elsevier Ltd. This is an open access article under the CC BY-NC-ND license (http://creativecommons.orgilicenses/by-nc-nd/4.0/).
引用
收藏
页码:97 / 106
页数:10
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