Magnetic Frustration, Phase Competition, and the Magnetoelectric Effect in NdFe3(BO3)4

被引:26
|
作者
Hamann-Borrero, J. E. [1 ]
Partzsch, S. [1 ]
Valencia, S. [2 ]
Mazzoli, C. [3 ,4 ,5 ]
Herrero-Martin, J. [5 ,6 ]
Feyerherm, R. [2 ]
Dudzik, E. [2 ]
Hess, C. [1 ]
Vasiliev, A. [7 ]
Bezmaternykh, L. [8 ]
Buechner, B. [1 ,9 ]
Geck, J. [1 ]
机构
[1] IFW Dresden, Leibniz Inst Solid State & Mat Res, D-01171 Dresden, Germany
[2] Helmholtz Zentrum Berlin, D-12489 Berlin, Germany
[3] Politecn Milan, I-20133 Milan, Italy
[4] Unita CNISM, I-20133 Milan, Italy
[5] European Synchrotron Radiat Facil, F-38043 Grenoble, France
[6] CSIC, Inst Ciencia Mat Barcelona, ICMAB, E-08193 Barcelona, Spain
[7] Moscow MV Lomonosov State Univ, Fac Phys, Low Temp Phys Dept, Moscow 119992, Russia
[8] Russian Acad Sci, Siberian Div, LV Kirensky Phys Inst, Krasnoyarsk 660036, Russia
[9] Tech Univ Dresden, Inst Solid State Phys, D-01062 Dresden, Germany
关键词
X-RAY-SCATTERING; POLARIZATION DEPENDENCE; EXCHANGE SCATTERING; MULTIFERROICS; BEAMLINE;
D O I
10.1103/PhysRevLett.109.267202
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We present an element selective resonant magnetic x-ray scattering study of NdFe3(BO3)(4) as a function of temperature and applied magnetic field. Our measurements show that the magnetic order of the Nd sublattice is induced by the Fe spin order. When a magnetic field is applied parallel to the hexagonal basal plane, the helicoidal spin order is suppressed and a collinear ordering, where the moments are forced to align in a direction perpendicular to the applied magnetic field, is stabilized. This result excludes a noncollinear spin order as the origin of the magnetically induced electric polarization in this compound. Instead our data imply that magnetic frustration results in a phase competition, which is the origin of the magnetoelectric response. DOI: 10.1103/PhysRevLett.109.267202
引用
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页数:5
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