A Double-Walled Bimetal-Organic Framework for Antibiotics Sensing and Size-Selective Catalysis

被引：55

作者：

He, Hongming ^{[1
]}

Xue, Ya-Qi ^{[1
]}

Wang, Shu-Qi ^{[1
]}

Zhu, Qian-Qian ^{[1
]}

Chen, Jing ^{[1
]}

Li, Cheng-Peng ^{[1
]}

Du, Miao ^{[1
]}

机构：

[1] Tianjin Normal Univ, Coll Chem, Tianjin Key Lab Struct & Performance Funct Mol, MOE Key Lab Inorgan Organ Hybrid Funct Mat Chem, Tianjin 300387, Peoples R China

来源：

INORGANIC CHEMISTRY | 2018年 / 57卷 / 24期

基金：

中国国家自然科学基金;

关键词：

GAS-ADSORPTION; SINGLE-CRYSTAL; BUILDING UNITS; METAL; MOF; CLUSTER; VERSATILE; LIGAND; STRATEGY; CAPTURE;

D O I：

10.1021/acs.inorgchem.8b01898

中图分类号：

O61 [无机化学];

学科分类号：

070301 ; 081704 ;

摘要：

The first double-walled bimetal-organic framework [Cd4K4(TADA)(4)(H2O)(12)]center dot 6DMF (1, TADA = 3,3'-((6-hydroxy-1,3,5-triazine-2,4-diyObis(azanediyl)) dibenzoate) has been successfully constructed. In virtue of its high porosity and abundant basic sites, MOF 1 can be served as a high-efficiently size-selective heterogeneous catalyst for Knovenagel condensation reaction. Remarkably, 1 also exhibits excellent luminescent detectability for metronidazole (MDZ) with the highest quenching constant (K-sv) of 1.16 X 10(5) M-1. The results demonstrate that 1 can be served as a unique bifunctional platform for antibiotics sensing and size-selective catalysis.

引用

页码：15062 / 15068

页数：7

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