Maximum reasonable radioxenon releases from medical isotope production facilities and their effect on monitoring nuclear explosions

被引:60
|
作者
Bowyer, Theodore W. [1 ]
Kephart, Rosara [1 ]
Eslinger, Paul W. [1 ]
Friese, Judah I. [1 ]
Miley, Harry S. [1 ]
Saey, Paul R. J. [2 ]
机构
[1] Pacific NW Natl Lab, Natl Secur Div, Richland, WA 99354 USA
[2] Austrian Univ, Vienna Univ Technol, Inst Atom, A-1020 Vienna, Austria
关键词
CTBT; Medical isotopes; Radioxenon; Nuclear explosion; TEST-BAN TREATY; XENON; SYSTEM;
D O I
10.1016/j.jenvrad.2012.07.018
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Fission gases such as Xe-133 are used extensively for monitoring the world for signs of nuclear testing in systems such as the International Monitoring System (IMS). These gases are also produced by nuclear reactors and by fission production of Mo-99 for medical use. Recently, medical isotope production facilities have been identified as the major contributor to the background of radioactive xenon isotopes (radioxenon) in the atmosphere (Stocki et al., 2005; Saey, 2009). These releases pose a potential future problem for monitoring nuclear explosions if not addressed. As a starting point, a maximum acceptable daily xenon emission rate was calculated, that is both scientifically defendable as not adversely affecting the IMS, but also consistent with what is possible to achieve in an operational environment. This study concludes that an emission of 5 x 10(9) Bq/day from a medical isotope production facility would be both an acceptable upper limit from the perspective of minimal impact to monitoring stations, but also appears to be an achievable limit for large isotope producers. (C) 2012 Elsevier Ltd. All rights reserved.
引用
收藏
页码:192 / 200
页数:9
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