Application of low-cost fine particulate mass monitors to convert satellite aerosol optical depth to surface concentrations in North America and Africa

被引:17
|
作者
Malings, Carl [1 ,2 ,6 ]
Westervelt, Daniel M. [3 ]
Hauryliuk, Aliaksei [4 ]
Presto, Albert A. [4 ]
Grieshop, Andrew [5 ]
Bittner, Ashley [5 ]
Beekmann, Matthias [1 ,2 ]
Subramanian, R. [1 ,2 ]
机构
[1] Univ Paris, Univ Paris Est Creteil, Ecole Natl Ponts & Chausses, CNRS UMS 3563,OSU EFLUVE Observ Sci Univers Envel, Paris, France
[2] Univ Paris, Univ Paris Est Creteil, Inst Pierre Simon Lapl, UMR 7583,CNRS,Lab Interuniv Syst Atmospher LISA, Creteil, France
[3] Columbia Univ, Lamont Doherty Earth Observ, New York, NY USA
[4] Carnegie Mellon Univ, Ctr Atmospher Particle Studies, 5000 Forbes Ave, Pittsburgh, PA 15213 USA
[5] North Carolina State Univ, Dept Civil Construct & Environm Engn, Raleigh, NC USA
[6] Goddard Space Flight Ctr, Greenbelt, MD 20771 USA
基金
美国安德鲁·梅隆基金会; 美国国家科学基金会;
关键词
GROUND-LEVEL PM2.5; LONG-TERM EXPOSURE; AIR-POLLUTION; ELECTROCHEMICAL SENSORS; CALIBRATION MODEL; GLOBAL MORTALITY; UNITED-STATES; MATTER; AMBIENT; QUALITY;
D O I
10.5194/amt-13-3873-2020
中图分类号
P4 [大气科学(气象学)];
学科分类号
0706 ; 070601 ;
摘要
Low-cost particulate mass sensors provide opportunities to assess air quality at unprecedented spatial and temporal resolutions. Established traditional monitoring networks have limited spatial resolution and are simply absent in many major cities across sub-Saharan Africa (SSA). Satellites provide snapshots of regional air pollution but require ground-truthing. Low-cost monitors can supplement and extend data coverage from these sources worldwide, providing a better overall air quality picture. We investigate the utility of such a multi-source data integration approach using two case studies. First, in Pittsburgh, Pennsylvania, both traditional monitoring and dense low-cost sensor networks are compared with satellite aerosol optical depth (AOD) data from NASA's MODIS system, and a linear conversion factor is developed to convert AOD to surface fine particulate matter mass concentration (as PM2.5). With 10 or more ground monitors in Pittsburgh, there is a 2-fold reduction in surface PM2.5 estimation mean absolute error compared to using only a single ground monitor. Second, we assess the ability of combined regional-scale satellite retrievals and local-scale low-cost sensor measurements to improve surface PM2.5 estimation at several urban sites in SSA. In Rwanda, we find that combining local ground monitoring information with satellite data provides a 40% improvement in surface PM2.5 estimation accuracy with respect to using low-cost ground monitoring data alone. A linear AOD-to-surface-PM2.5 conversion factor developed in Kigali, Rwanda, did not generalize well to other parts of SSA and varied seasonally for the same location, emphasizing the need for ongoing and localized groundbased monitoring, which can be facilitated by low-cost sensors. Overall, we find that combining ground-based low-cost sensor and satellite data, even without including additional meteorological or land use information, can improve and expand spatiotemporal air quality data coverage, especially in data-sparse regions.
引用
收藏
页码:3873 / 3892
页数:20
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