A novel estimate of the two-photon double-ionization cross section of helium

被引:14
|
作者
Malegat, L. [1 ]
Bachau, H. [2 ]
Piraux, B. [3 ]
Reynal, F. [2 ]
机构
[1] CNRS, Aime Cotton Lab, UPR 3321, F-91405 Orsay, France
[2] Univ Bordeaux 1, CNRS, CEA, Ctr Lasers Intenses & Applicat CELIA, F-33405 Talence, France
[3] Catholic Univ Louvain, Inst Condensed Matter & Nanosci IMCN, B-1348 Louvain, Belgium
关键词
Helium; -; Photons; Photoionization;
D O I
10.1088/0953-4075/45/17/175601
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
In a previous publication, a procedure was proposed for unambiguously extracting the cross sections for double ionization and single ionization from a time-propagated wavepacket, and it was tested on the well-known case of one-photon double ionization of helium successfully. Here, we apply it to the two-photon process for which the numerically predicted double ionization cross section is not completely stabilized yet. Our results confirm the value obtained for this cross section by all but two active groups in the field, they definitely exonerate electron correlations in the final state from any responsibility in this splitting of the published data into two sets, they emphasize the need for a more careful account of reflection effects and propose a tentative explanation for an overestimation of the cross section in the J-matrix method. They also demonstrate the conceptual and computational advantages of the method proposed.
引用
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页数:13
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