Hydrogen Production from Methane Steam Reforming in Combustion Heat Assisted Novel Microchannel Reactor with Catalytic Stacking

被引:13
|
作者
Lee, Chun-Boo [1 ,2 ]
Lee, Sung-Wook [1 ,2 ]
Lee, Dong-Wook [1 ]
Ryi, Shin-Kun [1 ]
Park, Jong-Soo [1 ]
Kim, Sung-Hyun [2 ]
机构
[1] Korea Inst Energy Res, Energy Mat & Convergence Res Dept, Taejon 305343, South Korea
[2] Korea Univ, Dept Chem & Biol Engn, Seoul 136701, South Korea
关键词
ETHANOL; MEMBRANE;
D O I
10.1021/ie402350a
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
In this study, we further investigate the application of an MCR containing a nickel metal catalyst with variable number of stacks for hydrogen production via MSR. Microchannels were contained in the MCR one side of the nickel metal catalyst with variable number of stacks for producing hydrogen to generate the necessary heat for the endothermic MSR and the combustion reaction was performed on the other side of the MCR The catalyst used in this study for the MSR reaction, which was a prepared Pd[0.1]-Al[0.3]/Ni catalyst. The methane conversion and hydrogen production mole ratio were 94.7% and 9.39 mol h(-1), respectively, and the steam/carbon (S/C) ratio was 3 at 650 degrees C, GHSV = 10 000 h(-1). The promise of a feasible simplified system for hydrogen production from the MSR was confirmed. If a hydrogen separation membrane is placed between the MSR elements in an MCR, the forward reaction will be preferentially promoted by the rapid removal of the hydrogen produced through the MSR reaction.
引用
收藏
页码:14049 / 14054
页数:6
相关论文
共 50 条
  • [1] Optimization of a counter-flow microchannel reactor using hydrogen assisted catalytic combustion for steam reforming of methane
    Jeon, Seung Won
    Yoon, Won Jae
    Jeong, Min Woo
    Kim, Yongchan
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2014, 39 (12) : 6470 - 6478
  • [2] Catalytic combustion assisted methane steam reforming in a catalytic plate reactor
    Zanfir, M
    Gavriilidis, A
    CHEMICAL ENGINEERING SCIENCE, 2003, 58 (17) : 3947 - 3960
  • [3] Hydrogen production in Multi-Channel Membrane Reactor via Steam Methane Reforming and Methane Catalytic Combustion
    Vigneault, Alexandre
    Grace, John R.
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2015, 40 (01) : 233 - 243
  • [4] Methane steam reforming in a novel ceramic microchannel reactor
    Murphy, Danielle M.
    Manerbino, Anthony
    Parker, Margarite
    Blasi, Justin
    Kee, Robert J.
    Sullivan, Neal P.
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2013, 38 (21) : 8741 - 8750
  • [5] Characteristic Investigation on the Methanol Steam Reforming Microchannel Reactor with the Novel Catalytic Combustion Self-Heating Structure for Hydrogen Production
    Ma, Ze-yu
    Li, Yuan
    Bao, Daorina
    Gao, Hong
    Cui, Wei
    INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2024, 63 (11) : 4782 - 4794
  • [6] Methane steam reforming thermally coupled with catalytic combustion in catalytic microreactors for hydrogen production
    Chen, Junjie
    Yan, Longfei
    Song, Wenya
    Xu, Deguang
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2017, 42 (01) : 664 - 680
  • [7] Experiments on hydrogen production from methanol steam reforming in the microchannel reactor
    Du, Xiaoze
    Shen, Yinqi
    Yang, Lijun
    Shi, Yingshuang
    Yang, Yongping
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2012, 37 (17) : 12271 - 12280
  • [8] Parametric study of methane steam reforming to syngas in a catalytic microchannel reactor
    Karakaya, Mustafa
    Keskin, Seda
    Avci, Ahrnet K.
    APPLIED CATALYSIS A-GENERAL, 2012, 411 : 114 - 122
  • [9] Transport characteristic study of methane steam reforming coupling methane catalytic combustion for hydrogen production
    Wang, Feng
    Zhou, Jing
    Wang, Guoqiang
    INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2012, 37 (17) : 13013 - 13021
  • [10] Heat-integrated reactor concepts for hydrogen production by methane steam reforming
    Kolios, G
    Glöckler, B
    Gritsch, A
    Morillo, A
    Eigenberger, G
    FUEL CELLS, 2005, 5 (01) : 52 - 65