High-field ESR Studies of the Quantum Spin Dimer System Ba3Cr2O8

被引:9
|
作者
Kamenskyi, D. [1 ]
Wosnitza, J. [1 ]
Krzystek, J. [2 ]
Aczel, A. A. [3 ,4 ]
Dabkowska, H. A. [3 ]
Dabkowski, A. B. [3 ]
Luke, G. M. [3 ]
Zvyagin, S. A. [1 ]
机构
[1] Helmholtz Zentrum Dresden Rossendorf, Dresden High Magnet Field Lab HLD, D-01328 Dresden, Germany
[2] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA
[3] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada
[4] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA
关键词
Electron spin resonance; Field-induced phase transition; Dimers; SRCU2(BO3)(2); TLCUCL3; STATE;
D O I
10.1007/s10909-012-0722-4
中图分类号
O59 [应用物理学];
学科分类号
摘要
Results of systematic high-frequency electron spin resonance (ESR) studies of Ba3Cr2O8, a weakly coupled dimer system, in magnetic fields up to 25 T are reported. Two pairs of ESR gapped modes corresponding to transitions from a spin-singlet ground state to the first excited triplet states with gaps, Delta (AB) =563 GHz and Delta (CD) =399 GHz, are revealed below H (c1)=12.5 T. The detection of the ground-state excitations by means of ESR clearly indicates the presence of a non-secular term allowing these transitions. A complex structure of the microwave absorption spectrum in magnetic fields above H (c1) is observed, those peculiarities are discussed.
引用
收藏
页码:231 / 235
页数:5
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