Hydrogen production by natural gas in a compact ATR-based kW-scale fuel processor

被引:5
|
作者
Palma, Vincenzo [1 ]
Ricca, Antonio [1 ]
Addeo, Biagio [1 ]
Rea, Maurizio [2 ]
Paolillo, Gaetano [2 ]
Ciambelli, Paolo [1 ]
机构
[1] Univ Salerno, Dept Ind Engn, Via Giovanni Paolo 2 132, I-84084 Fisciano, SA, Italy
[2] SOL Spa, Via Borgazzi 27, I-20052 Monza, MI, Italy
关键词
Fuel processor; Distributed hydrogen production; Thermal integration; PARTIAL OXIDATION; REFORMING PROCESS; METHANE; CATALYSTS; PERFORMANCE; REACTOR; CELLS; SUPPORT; DESIGN; SYNGAS;
D O I
10.1016/j.ijhydene.2016.06.049
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In the present work, the design and testing of a very compact reaction system thermally integrated for the distributed hydrogen production by natural gas reforming is reported. The system is based on hydrocarbon Auto-Thermal Reforming, followed by a Water-Gas Shift module. A compact heat exchanger was placed between the two catalytic stages, in order to assure an appropriate thermal integration, thus avoiding any other external heat duties. Experimental results demonstrated that the integrated configuration assured a good management of thermal fluxes in the system, in which an effective heat recovery from ATR exhaust gas to reactants was realized. Preliminary tests showed very impressive performances of the system, both by processing methane and natural gas. Despite a quite inefficient WGS stage, the processor was able to produce up to 10 Nm(3)/h of hydrogen, assuring a thermal efficiency higher than traditional systems. (C) 2016 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:1579 / 1589
页数:11
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