Alpha spectrometry isotopic ratios indications in the Paleozoic sedimentary rock of El Gor area, Southwestern Sinai, Egypt: insights on uranium mobility age

被引:3
|
作者
Khattab, Mahmoud R. [1 ]
机构
[1] Nucl Mat Author NMA, Geochem Explorat Dept, POB 530, Cairo, Egypt
关键词
Radionuclides; alpha spectrometry; radiochemistry; uranium isotopes; thorium isotopes; SAMPLES;
D O I
10.1080/10934529.2023.2165865
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The study area is located between longitude 33 degrees 18' 00" - 33 degrees 21' 00" E and latitude 28 degrees 59' - 29 degrees 01' N and covers approximately 700km(2). Uranium and thorium isotopes were determined by alpha spectrometry. The activity concentrations of U-238, U-234 and U-235 were ranged between 245.5 +/- 8.3-465.2 +/- 15.2 Bq.kg(-1) with an average 345.5 +/- 10.4-452.5 +/- 9.3 Bq.kg(-1) and 890.5 +/- 21.3 Bq.kg(-1) with an average 632.3 +/- 14.9-11.40 +/- 0.5 Bq.kg(-1) and 21.50 +/- 1.4 Bq.kg(-1), respectively. The activity concentration of Th-232, Th-230 and Th-228 were ranged between 153.1 +/- 0.3-318.1 +/- 2.9 Bq.kg(-1), 149.5 +/- 0.7-280.8 +/- 2.2 Bq.kg(-1) and 36.9 +/- 0.1-60.5 +/- 0.9 Bq.kg(-1). The Th-230/Th-232 activity ratios in all samples were lower than 20, indicating that these samples have been contaminated by detrital Th-230. Th/U ratio varied between 1.3 and 2.1 with an average 1.8; all values were lower than 3.5, indicated enrichment of uranium. U-234/U-238 activity ratios that higher than unity indicates that an isotope of uranium has migrated within the rock. From the isotopes of uranium and thorium and their activity ratios, the isochron age for the collected samples was about 58.96 ka.
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页码:424 / 432
页数:9
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