DEPENDENT ELECTRON TRANSMISSION;
MOLECULES;
SELECTIVITY;
D O I:
10.1063/5.0156316
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
Chirality-induced spin selectivity has been reported in many experiments, but a generally accepted theoretical explanation has not yet been proposed. Here, we introduce a simple model system of a straight cylindrical free-electron wire containing a helical string of atomic scattering centers with spin-orbit interaction. The advantage of this simple model is that it allows deriving analytical expressions for the spin scattering rates, such that the origin of the effect can be easily followed. We find that spin-selective scattering can be viewed as resulting from the constructive interference of partial waves scattered by the spin-orbit terms. We demonstrate that forward scattering rates are independent of spin, while back scattering is spin dependent over wide windows of energy. Although the model does not represent the full details of electron transmission through chiral molecules, it clearly reveals a mechanism that could operate in chiral systems.
机构:
Univ Cambridge, Dept Mat Sci & Met, Cambridge CB3 0FS, EnglandUniv Cambridge, Dept Mat Sci & Met, Cambridge CB3 0FS, England
Robinson, J. W. A.
Samokhvalov, A., V
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机构:
Russian Acad Sci, Inst Phys Microstruct, GSP 105, Nizhnii Novgorod 603950, Russia
Lobachevsky State Univ Nizhni Novgorod, 23 Prospekt Gagarina, Nizhnii Novgorod 603950, RussiaUniv Cambridge, Dept Mat Sci & Met, Cambridge CB3 0FS, England
Samokhvalov, A., V
Buzdin, A., I
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机构:
Univ Cambridge, Dept Mat Sci & Met, Cambridge CB3 0FS, England
Univ Bordeaux, LOMA UMR CNRS 5798, F-33405 Talence, France
Sechenov First Moscow State Med Univ, Moscow 119991, RussiaUniv Cambridge, Dept Mat Sci & Met, Cambridge CB3 0FS, England
机构:
Korea Adv Inst Sci & Technol, Dept Biol Sci, Daejeon 34141, South KoreaKorea Adv Inst Sci & Technol, Dept Biol Sci, Daejeon 34141, South Korea
Lee, Juhee
Jung, Wookjin
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Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Daejeon 34141, South KoreaKorea Adv Inst Sci & Technol, Dept Biol Sci, Daejeon 34141, South Korea
Jung, Wookjin
Lee, Dongkyu
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Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Daejeon 34141, South KoreaKorea Adv Inst Sci & Technol, Dept Biol Sci, Daejeon 34141, South Korea
Lee, Dongkyu
Kang, Mihyun
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机构:
Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Daejeon 34141, South KoreaKorea Adv Inst Sci & Technol, Dept Biol Sci, Daejeon 34141, South Korea
Kang, Mihyun
Chung, Hyun Jung
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Korea Adv Inst Sci & Technol, Dept Biol Sci, Daejeon 34141, South KoreaKorea Adv Inst Sci & Technol, Dept Biol Sci, Daejeon 34141, South Korea
Chung, Hyun Jung
Yeom, Jihyeon
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Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Daejeon 34141, South KoreaKorea Adv Inst Sci & Technol, Dept Biol Sci, Daejeon 34141, South Korea
机构:
JNCASR, New Chem Unit, Supramol Chem Lab, Bangalore 560064, Karnataka, IndiaJNCASR, New Chem Unit, Supramol Chem Lab, Bangalore 560064, Karnataka, India
Sarkar, Aritra
Dhiman, Shikha
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JNCASR, New Chem Unit, Supramol Chem Lab, Bangalore 560064, Karnataka, IndiaJNCASR, New Chem Unit, Supramol Chem Lab, Bangalore 560064, Karnataka, India
Dhiman, Shikha
Chalishazar, Aditya
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机构:
JNCASR, New Chem Unit, Supramol Chem Lab, Bangalore 560064, Karnataka, IndiaJNCASR, New Chem Unit, Supramol Chem Lab, Bangalore 560064, Karnataka, India
Chalishazar, Aditya
George, Subi J.
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机构:
JNCASR, New Chem Unit, Supramol Chem Lab, Bangalore 560064, Karnataka, IndiaJNCASR, New Chem Unit, Supramol Chem Lab, Bangalore 560064, Karnataka, India
机构:
Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA
Univ Tokyo, Inst Phys & Math, Kashiwa, Chiba 2778568, JapanUniv Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
Buckley, Matthew R.
Murayama, Hitoshi
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机构:
Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA
Univ Tokyo, Inst Phys & Math, Kashiwa, Chiba 2778568, JapanUniv Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
Murayama, Hitoshi
Klemm, William
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机构:
Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
Univ Tokyo, Inst Phys & Math, Kashiwa, Chiba 2778568, JapanUniv Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
Klemm, William
Rentala, Vikram
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机构:
Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA
Univ Tokyo, Inst Phys & Math, Kashiwa, Chiba 2778568, JapanUniv Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA